Monitoring black carbon concentrations with mobile devices ... · Extra bikersand commuters 5...
Transcript of Monitoring black carbon concentrations with mobile devices ... · Extra bikersand commuters 5...
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Monitoring black carbonconcentrations with mobile devices in the city of Liège
L. Bertrand, F. Lenartz, F. Detalle, N. Fernemont (ISSeP)
C. Louis, Y. Cornet (University of Liège)
EFCA – Ultrafine Particles – Brussels 4‐5 May 2015
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CONTEXTInitiative of ISSeP
Interaction soughtwith city of Liège (nb: streetcar to partly replace buses)
EC encourages BC monitoring
Wallonia/ISSeP:3 analysers (fixednetwork) + mobile analysers in trailers
0% 50% 100%
Marchienne
Herstal
Vielsalm
PM2.5
PM10‐PM2.5
0 10 20 30
Marchienne
Herstal
Vielsalm
PM2.5
PM10‐PM2.5
http://193.190.182.213/WebAirQuality/MicroParticules.aspx
0% 20% 40% 60% 80% 100%
Marchienne
Herstal
Vielsalm
BC
PM10‐BC
2
PMx µg/m³rural background
urban‐industrial
industrial
PM2,5 vs coarserural background
urban‐industrial
industrial
PM2,5 vs coarserural background
urban‐industrial
industrial
Walloon BC data, April 2011 to end 2014Int 1/6
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Definition : form of particulate matter which captures most efficiently solar energy [EPA]
Source :Incomplete combustion of fossil fuels [EEA]
Noxiouxness :Hazard at least as important as that of PM2,5 [WHO]
Measurement (in Wallonia)AE 22 aethalometersAE51 aethalometers
Black Carbon
Transmission electron microscopy (TEM) images of aerosolparticles, including black carbon from Posfai et al. (1999). In panelA, the black carbon particles (denoted by the small arrows) aremixed with inorganic ammonium sulphate particles. In panel B, atypical chain‐like black carbon aggregate is shown with the arrowspointing to a film of carbon that connects the individual spheruleswithin the aggregate. In panel C, fly‐ash spheres are shown, whichare particles that are often associated with black carbon particles.
Int 2/6
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Analysers in use: Magee scientific AE22 Aethalometer – 2 wavelenghs
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ruralbgrd
urbanindust ind.
Int 3/6
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BC patters at urban‐industrial station µg/m³
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→ peaks correspond to trafic (rush hours)→ higher values in winter months
saturday
sunday
rush hours
Int 4/6
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Components of the ExTraCar project
Measurement, mapping, spatial and temporal characterisation of BC levelsin the city of Liège . . .(cf issues in Liège, streetcar on track)
Modelling of BC levels :towards decision oriented tools for local authorities
Assesment of Exposure of commuters during their trip (greater Liège area)
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Int 5/6
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team within ISSePCore from Air Quality UnitF. Lenartz, L. BertrandF. Detalle, Fernemont
Application developpersA. Caprioli (DB), P. Crespin (GIS)
Extra bikers and commuters5 colleagues
Brussels‐EnvironmentO. Brasseur, P. Declerck,
University of Liège‐ Geomatics
Y. Cornet
Universiteit Hasselt‐ IMOBD. Janssens
StudentsS. Tchiaye‐Dongmo (IMOB)C. Louis (ULg)I. Elghazi (Univ‐Meknès)
partners/assistance
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Int 6/6
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ExTraCar: mobile equipment: bikers
6 Black CarbonAE51
GPS GlobalSatDG‐200
Grimm 1109
1 wavelenth880 nm
Does’nt sendData
downloadedPM10‐PM2,5‐
PM1
8
Gps
AE51
Grimm1109
Methods 1/6
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2. First loops and experiencesselected track n°73 18/04/2013 from 14h05 BC
Green areas,bikers and pedestrian lanes
Busy streetsand squares
BC levelsng/m³
automaticcolorscale
web‐gis application, one loop to begin withMethods 2/6
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Actual commuting track
Yves Cornet, home
Geomatics,ULg
Liège
with electrical bike ~22 km
~70 m
~270 m
Methods 3/6
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Train station
Place St‐LambertBressoux5,9 km
Citadelle 5,8 km
Chenée5,9 km
Sclessin6,7 km
Louvrex6,7 km
Médiacité5,8 km
6 loops chosen to map concentrationsin the city
5 of 6 pass either in front of train station or at Saint‐Lambert
In each loop bothbusy/canyon streetsand open/green parts
biker:3 to 4 timesa loop
[Measurementsmorning of afternoonrushHours,mainly]
Loops chosenin LiègeMethods 4/6
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web-gis
Louvrex,15h40
Médiacité,15h40
Bressoux,15h57
one track displayedfor each loop ,
tracks 404,405,406
BCConcµg/m³
Methods 5/6
Loops 12/03/2015
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Herstal (Fabian)
ISSeP
Train+ walking
Bike
Car
Commuter’s exposure: Train, Car, BikeMethods 6/6
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Observed errors in tracker’s records
Wrong positioningaway from trackand along track
no records (signal loss)
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Simple casesStudent’s master
thesis
Gps data processingData 1/7
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More complex caseActual bike lane
Gps recorded track
Gps
Data 2/7
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sophisticated /Expensive gps . . . the six DG 200
no benefit from using other devicefor the data correction procedures
the project will stick with the simple tracker chosen
Gps trackersLoop done with→ expensive GPS→ our six DG200
UNCERTAINTIES, 1 sec synchronisation error(analyser versus gps tracker) :
walking: discrepancy 1.11 m (4 kmh‐1) biking: discrepancy : 5.55 m (20 kmh‐1) car……………… tracker precision: typically 10 m
Data 3/7
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14% 4% 3%0
1
2
3
4
5
6
7
09/09/14 27/10/14 28/11/14
trial mean
Comparisons of the six AE51 (µg/m³)at the Herstal automatic station
→ The precision improves with higher concentrations
Data 4/7
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raw 1 sec 10 sec centered 30 sec centered
how to best process AE51 1 sec results ?
1000 1200 1400 1600 1800 2000 2200
-5
0
5
10
15
20
25
30
35
Time (s)
BC
(µg/
m3)
RAWCRM 10sCRM 30sCRM 60s
60 sec centered*
Data 5/7
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SIX moving AE51 compared, running mean or rather running median ?
→running median chosen, less inter‐instrument discrepancies
16:00 17:00 18:00 19:00-5
0
5
10
15
20
25
Date: 25/09/14
BC
[µgm
-3]
C.R.Mean data
16:00 17:00 18:00 19:00-5
0
5
10
15
20
Date: 25/09/14
BC
[µgm
-3]
C.R.Median data
AE1AE2AE3AE4AE6AE8
Mean: discrepancies
Median: it’s better
16h00 18h00
Data 6/7
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1st AE51: 1 sec time step2nd AE51: 1 min time step
TRAINMean AE1 (sec): 1973Mean AE2 (min) 2028
BIKEMean AE4: 1790Mean AE6: 1855
BC [ngm-3]1 min mean * 1 min result (2nd device)
BikerTrain passenger each
reasonable agreement between1 min mean and 1 min result
All 4 AE51Colocatedat Fabian’s
∆ 2,7%
∆ 3,6%
ISSeP16h55
Herstal, Fabian home 18h10
experience done on communting tracks
train
bike
Data 7/7
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Needs for regional model; meteo data, continuous monitoring
ExTraCar BC analysers
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St‐Lambert
ISSeP
Modelling 1/7
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Street Model : application planned for 6 streets
Figures drawn from the report Modelling traffic pollution in streets published by the Danish National Environmental Research Institute and the Ministry of Environmentand Energy
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Use of the model adapted for BC by partner Brussels‐Environment~ algorithms similar to OSPM
Modelling 2/7
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Trafic source‐ TRAFIC DATA ‐ → 2010‐2011 annual km, city area,
Highway/Urban/(rural) – Long/Short vehiculesFrom AwAC (Walloon inventories)
‐ → Noise study of 2012 : ~ 70 sites , one day data (1 hour resolution)‐ → Buses: data from bus operator TEC‐Liège‐ → ExTraCar oswn counts: 6 chosen streets (application of street model)
‐ EMISSION FACTORS (BC now available (EEA/EMEP +HBEFA)‐ → official 2015 walloon factors‐ → adjustment related to measurements foreseen
Modelling 3/7
References:Modelling black carbon concentrations in two busy street canyons in Brussel using CANBCAtmosenv, 101 (2015),, O. Brasseur and al + + mail O. Brasseur 17/03/2015Modfelling the effect of speed limit reduction on trafic related elemental carbon (EC) concentrations and population exposureto BC, Wouter Lefebvre and al, Atmoasenv, 45 (2011)
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Radar (24h)ManualPolice
2012 counting sites (noise study) ExTraCar counting sites
Modelling 4/7
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2
1
2
1
2
2+ 2bus
The 6 ExTraCar counting sites + number of ways/lanesModelling 5/7
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ExTraCar counting‐ use of two radar TMS‐SA4 lent by DGO1‐52 of SPW‐ began 27/04/2012‐ cross check with manual countings (at rush hours)
→ BC measurement boths by bikers and counters duringthe manual counting sessions
also consistency check with recieved existing data
Pictures:
manufacturer
Modelling 6/7
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From AwAC, performing Walloon Emission inventories‐ ‐ Number of houselholds using the various fossil fuelsFrom PIC: space disagregated volume of dwellings, service activitesTime desagregation taking outdoor temperatures into account
Modelling 7/7 Domestic heating
Sources : P. Théate, D. Derriks and X. Frippiat from AwAC (Agence wallonne de l’Air et du Climat)EMEP/EEA emission inventory guidebook 2013
Emission factors for TSPEFTSP [mg/GJ]
log scale:→ Only some fossilfuels matter
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Advancement 1/3 Meteo representativeness: loops
Morning rush Evening rush Other times
Stability class Stable Neutral Unstable Stable Neutral Unstable Stable Neutral Unstable
Loops as03/04/2015 T G T G T G T G T G T G T G T G T G
Chênée ? 8 ? 0 ? 0 ? 4 ? 10 ? 0 / 0 / 4 / 0
Bressoux ? 9 ? 11 ? 0 ? 7 ? 26 ? 0 / 0 / 13 / 0
Citadelle ? 10 ? 3 ? 0 ? 4 ? 11 ? 0 / 0 / 1 / 0
Louvrex ? 18 ? 11 ? 0 ? 3 ? 34 ? 0 / 0 / 16 / 0
Médiacité ? 13 ? 3 ? 0 ? 4 ? 36 ? 0 / 0 / 11 / 0
Sclessin ? 11 ? 3 ? 0 ? 4 ? 15 ? 0 / 0 / 1 / 0
T = target; G: results actually gotThe purpose is to get for each loop data , data spread as evenly as possiblein the three main stability classes and betwenn morning and evening rushAs April 3rd, 2015, we had’nt yet encountered Unstable conditions for the loops
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Meteo representativeness: commuting tripsAdvancement 2/3
Morning rush Evening rushStability class Stable Neutral Unstable Stable Neutral Unstable
Trips as 03/04/2015 T G T G T G T G T G T G
Herstal ‐ ISSePbike‐train‐car 3 3 3 3 3 0
ISSeP – Herstalbike‐train‐car 3 0 3 2 3 2
Herstal – ISSePbike‐train‐car+bus 3 2 3 0 3 0
ISSeP – Herstalbike‐train‐car+bus 3 0 3 1 3 0
Soumagne – ISSePbike‐bus‐car 3 1 3 1 3 2
ISSeP – Soumagnebike‐bus‐car 3 0 3 2 3 1
T = target; G: results actually got
Unstable consitions encountered, yet underrepresented
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Stability classes, issuesAdvancement 3/3
Daytime insolation Night‐time conditions
Surface wind speed (m/s) Strong Moderate Slight
Thin overcast or > 4/8 low cloud
<= 4/8 cloudiness
< 2 A A ‐ B B E F
2 ‐ 3 A ‐ B B C E F
3 ‐ 5 B B ‐ C C D E
5 ‐ 6 C C ‐ D D D D
> 6 C D D D D
PasquillClass
Sigma Theta(degrees)
Delta T/Delta Z (Deg C/100 m)
A 25 ‐1.9
B 20 ‐1.9 to ‐1.7
C 15 ‐1.7 to ‐1.5
D 10 ‐1.5 to ‐0.5
E 5 ‐0.5 to 1.5
F 2.5 1.5 to 4.0
G 1.7 >4.0
from http://www.ready.noaa.gov/READYpgclass.php
A: Extremely unstableB: Moderately unstable
D: NeutralE: Slightly stable
F: Moderately stableG: Extremely stable
The spread of stabilities in each scheme is large and sometimes it covers the entire range of stabilities for a given Pasquill class. However, it has been observed that the schemes based on Monin‐Obukov length and Richardson number gives (more*) reasonable comparison than the rest of the schemes. (…) The implications of this on estimated distance to maximum ground level concentrations are great and could affect the overalloutcome of conventional Gaussian models for industrial sitting, planning and management.
Manju Mohan and T.A. Siddiqui (1998), Analysis of various schemes for the estimation of atmospheric stability classification, Atmospheric Environment, Vol. 32, No. 21, pp. 3775‐3781
Clarification on this needed, to precise results still needed
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ComplianceMonitoring Network Theoretical Exposure
Engis
Jemeppe St‐Nicolas
ISSePChéra
Angleur
http://pmlab.irceline.beMean PM10 24h au 3 october 2014 at 5H00Values at monitoring sites + sophisticated interpolation 1 km gridExposure of somebody who would stay in front of home
Herstal Coronmeuse
Engis
Jemeppe St‐Nicolas
ISSePChéra
Angleur
Herstal Coronmeuse
Exposure 1/8
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APHEIS study, Public Heath Impact of PM10Brussels + Antwerp + Liège by ISSeP + KUL
Theoretical PM10 Exposure, reference year 2004Population dansity taken intoaccount, Estimationof health
effects
+
32
Exposure 2/8
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4 ISSeP persons (3 Lg, 1 Colf) Black Carbon (ng/m³)means of each person, 3+4 juin 2014Brussels‐Environment procedure with activity diaries
Fabian Isabelle Marie Luc
c cL r
Peaks
L leaving ISSeP during lunchtime
c commuting to, from work
r riding in the car in the evening
Exposure 3/8
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BC Exposure, one day details
Train + walking,Flémalle to Liège
at ISSeP out of buildings
Highwaytunnel E25‐E40
VisitGrivegnéecar
34
Train + walking,Liège to Flémalle
Exposure 4/8
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1 Herstal issep
a. bike b. train
2 Soumagne
issep
a. bike b. busc. car
3
1a
1b 1c
2a
2b
2c
Exposure of subjects while communting
CA ETC – 08/10/201435
c. car
Exposure 5/8
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ravel= completed separate bike routeLosses of gps signal for the bus passengerHot spots are visible
BC exposure while commuting
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Soumagne‐issep, 30/06/2014, bike, bus and car
car
bus
bike
Exposure 6/8
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BC Exposure while commutingExposure 7/8
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BC Exposure while commuting
! Here 3x Soumagne-issep et 1x issep-SoumagneExemple favourable for the biker
separated bike route for a significant part of the trip3 x downhill, 1 x uphill
Exposure 8/8