ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall...

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Chiara Ciccarelli University of Cambridge SPICE workshop on anti-ferromagnetic spintronics 26-30 September 2016 ZERO-MAGNETISATION SPIN-SOURCES

Transcript of ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall...

Page 1: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

Chiara CiccarelliUniversity of Cambridge

SPICEworkshoponanti-ferromagneticspintronics26-30September2016

ZERO-MAGNETISATIONSPIN-SOURCES

Page 2: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

Spin-Halleffectinanti-ferromagnets Element-selectivespin-emission

Spin-pumpingfromananti-ferromagnet

1

3

2

ZEROMAGNETISATIONSPIN-SOURCES

Page 3: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

EXPERIMENT1TheSpin-Halleffectinanti-ferromagnets

Page 4: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

xy

z

NiFe (4nm)

IrMn (4nm)Seedlayer

𝐦

Wedeterminethecurrent-inducedfieldsbyFMR

θ B

Page 5: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

xy

z

NiFe (4nm)

IrMn (4nm)Seedlayer

𝐦

Wedeterminethecurrent-inducedfieldsbyFMR

θ B

Vdc

V t = R ωt ×I ωt =

=V)* + V(2ωt)

Tulapurkar,Nature2005Fang,NatureNano2011

Page 6: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

xy

z

NiFe (4nm)

IrMn (4nm)Seedlayer

𝐦

θ B

Vdc

hz 1.13∓0.05mT

hy 1.04∓0.03mT

hOe 1.09∓0.07mT

@107 A/cm2

𝐡𝐳~𝛔×𝐦

Wedeterminethecurrent-inducedfieldsbyFMR

hyhz

Tshitoyan,PRB2015

Page 7: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

SHE-STTorELSE?

seedIrMn (4nm)

NiFe (4nm)Cu(2nm)

qSH(Ir20Mn80)∼0.8qSH(Pt)Mendes,2014q(Ir50Mn50)∼2% Zhang,2014

qSH =5.6%

Tshitoyan,PRB2015

Page 8: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

SHE-STTorELSE?

qSH =22%

Tshitoyan,PRB2015

seedIrMn (4nm)

NiFe (4nm)Cu(2nm)

seedIrMn (4nm)

NiFe (4nm)

Page 9: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

TheSHangleiscorrelatedtotheexchangefield

qSH =22%

Tshitoyan,PRB2015

Page 10: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

Coupleddynamicsmightbeattheoriginoftheincreaseinhz

µ>𝛻H ω = µ>𝛻HABC + αEFFωγ

Tshitoyan,PRB2015

Page 11: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

Coupleddynamicsmightbeattheoriginoftheincreaseinhz

µ>𝛻H ω = µ>𝛻HABC + αEFFωγ

WegetanegativevalueofGmixUnphysical

αEFF = αHI + αEJTshitoyan,PRB2015Tserkovnyak,PRB2002

Page 12: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

EXPERIMENT2Element-selectivespinemissionfroma

ferrimagnet

Page 13: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

Ultra-fastspinemissioninmagneticbilayers

Inthiscasetheemittedspincurrentisalignedwiththenetmagnetisation.

Isitpossibletohavezero-magnetisationspintronicemittersofTHzradiation?

T.Seifertetal.,NaturePhotonics2016T.Kampfrath etal.,NatureNanotech.2013

Page 14: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

3d-4falloys

Page 15: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

C.D.Stanciu etal.,PRB2006J.Becker,PhDthesis,2016

3d-4falloys

Page 16: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

150 200 250 3000

20

40

60

80

Mag

netis

atio

n (e

mu/

cm3 )

Temperature (K)

SiN(5nm)

Pt(2nm)Gd25Fe65.6Co9.4(20nm)

SiN(5nm)

EASYAXIS

Glass

Temperature(K)0100200300400 500600700

M(Gd)

M(Fe)

GdFeCo hasacompensationtemperatureatwhichM=0

Page 17: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

800nm50fs

zL

E(t) ≈ σAI(t)×zL

WeuseTHzemissionspectroscopytomeasurespin-emission

Page 18: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

446 447 448 449 450

-20

0

20

S(t)

(10-

6 )

time (ps)

2T -2T

ROOMTEMPERATURE

446 447 448 449 450 451

-20

-10

0

10

20

S(t)

(10-

6 )

time (ps)

0.5 from glass side 0.5 from GdFeCo side

𝛔𝐢𝐩(𝐭)

𝛔𝐢𝐩(𝐭)

BB

ThemittedTHzradiationhasthesymmetryoftheISHE

B B

𝛔𝐢𝐩(𝐭) 𝛔𝐢𝐩(𝐭)

Page 19: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

-2 -1 0 1 2-50

-40

-30

-20

-10

0

10

20

30

40

50

S(t)

(10-

6 )

B (T)

150 K 280 K

B

BELOWTcomp

B

ABOVETcomp

ThemittedTHzradiationissensitivetotheFespinonly

Gd

Fe

Gd

Fe

Page 20: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

-2 -1 0 1 2-50

-40

-30

-20

-10

0

10

20

30

40

50

S(t)

(10-

6 )

B (T)

150 K 160 K 170 K 180 K 190 K

ThemittedTHzradiationissensitivetotheFespinonly

E = −MUB sin θ1 −M\B sin θ2 + JMUM\ cos θ1 + θ2 −

−K2MU\ cos\ θ −

K2M\\ cos\ φ

𝐌𝟏

𝐌𝟐

Page 21: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

EXPERIMENT3Spin-pumpingfromanti-ferromagnets

Page 22: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

FERROMAGNETS

Spin-pumpingfromanAFM

R.Chengetal.,PRL2014

ANTI-FERROMAGNETS

Page 23: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

FERROMAGNETS

Spin-pumpingfromanAFM

R.Chengetal.,PRL2014

ANTI-FERROMAGNETS

100010

001

KNiF3

TN=246KEg=6.2eV

D.Bossini etal.,PRB2014

Page 24: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

FERROMAGNETS

Spin-pumpingfromanAFM

R.Chengetal.,PRL2014

ANTI-FERROMAGNETS

D.Bossini etal.,PRB2014

Page 25: ZERO-MAGNETISATION SPIN-SOURCES · ZERO MAGNETISATION SPIN-SOURCES. EXPERIMENT 1 The Spin-Hall effect in anti-ferromagnets. x y z NiFe(4 nm) IrMn (4 nm) Seed layer! We determine the

Spin-Halleffectinanti-ferromagnets Element-selectivespin-emission

Spin-pumpingfromananti-ferromagnet

SUMMARY

CambridgeVahe TshytoyanAndrewIrvineAndrewFerguson

LeedsTomMooreAndreiMihai,MannanAli

PragueTomasJungwirth

1

3

2

NijmegenAlexeyKimelThomasHuismanRostislav MikhaylovskiyTheoRasing

NijmegenAlexeyKimelThomasHuismanRostislav MikhaylovskiyTheoRasing

UniversityofTokyoDavide BossiniPragueZbynek SobanTomasJungwirth

LeedsTomMooreRowanTempleChrisMarrowsNottinghamAndrewRushforthBryanGallagher