Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting...

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Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions of Atmospheric Mercury at the Cape Hedo Atmosphere and Aerosol Monitoring Station (CHAAMS), Japan A. Yamakawa a , A. Takami b , Y. Takeda b , S. Kato c , Y. Kajii d,b a Center for Environmental Measurement and Analysis, National Institute for Environmental Studies, 16-2 Onogawa, Tsukuba 305-8506, Japan. b Center for Regional Environmental Research, National Institute for Environmental Studies, 16-2 Onogawa, Tsukuba 305-8506, Japan. c Department of Applied Chemistry for Environment, Faculty of Urban Environmental Sciences, Tokyo Metropolitan University, Minamiosawa 1-1, Hachioji, Tokyo 192-0397, Japan. d Graduate School of Global Environmental Studies, Kyoto University, Yoshida- Honmachi, Sakyo-ku, Kyoto 606-8501, Japan. Contents of this file 1. Figure S1. A GEM sampling system 2. Figures S2. Air-mass back trajectories of 24-h duration 3. Table S1 4. Figure S3. Ox concentrations at the monitoring stations Electronic Supplementary Material (ESI) for Environmental Science: Processes & Impacts. This journal is © The Royal Society of Chemistry 2019

Transcript of Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting...

Page 1: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

Supporting Information to:

Investigation of Mercury Emission Sources Using Hg Isotopic Compositions of Atmospheric Mercury at the Cape Hedo Atmosphere and Aerosol Monitoring Station (CHAAMS), Japan

A. Yamakawaa, A. Takamib, Y. Takedab, S. Katoc, Y. Kajiid,b

aCenter for Environmental Measurement and Analysis, National Institute for

Environmental Studies, 16-2 Onogawa, Tsukuba 305-8506, Japan.

bCenter for Regional Environmental Research, National Institute for Environmental

Studies, 16-2 Onogawa, Tsukuba 305-8506, Japan.

cDepartment of Applied Chemistry for Environment, Faculty of Urban Environmental

Sciences, Tokyo Metropolitan University, Minamiosawa 1-1, Hachioji, Tokyo 192-0397,

Japan.

dGraduate School of Global Environmental Studies, Kyoto University, Yoshida-

Honmachi, Sakyo-ku, Kyoto 606-8501, Japan.

Contents of this file

1. Figure S1. A GEM sampling system

2. Figures S2. Air-mass back trajectories of 24-h duration

3. Table S1

4. Figure S3. Ox concentrations at the monitoring stations

Electronic Supplementary Material (ESI) for Environmental Science: Processes & Impacts.This journal is © The Royal Society of Chemistry 2019

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Figure S1: A GEM sampling system. For avoiding breakthrough of GEM across the trap, the air flow rate was adjusted to 1.0 L/min per trap. In order to measure Hg isotopes with the required accuracy, >10 ng of GEM was necessary. Two Au traps were set parallel, and eight rows were prepared for the long term monitoring. The automatic switching valve was set to switch every 72 hours.

Quartz fiber and soda lime

Automatic switching valve

Air

Au traps

Air pump (1.0 L/min)

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Job ID: 187556 Job Start: Mon Oct 1 23:58:34 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 19 Dec 2016 - GDAS0p5

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Job ID: 187584 Job Start: Tue Oct 2 00:00:38 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 21 Dec 2016 - GDAS0p5

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Job ID: 187625 Job Start: Tue Oct 2 00:03:03 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 24 Dec 2016 - GDAS0p5

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Figure SI 2. Air-mass back trajectories of 24-h duration
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Job ID: 187633 Job Start: Tue Oct 2 00:03:54 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 25 Dec 2016 - GDAS0p5

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Job ID: 187769 Job Start: Tue Oct 2 00:08:19 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 29 Dec 2016 - GDAS0p5

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Job ID: 187823 Job Start: Tue Oct 2 00:09:23 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 30 Dec 2016 - GDAS0p5

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Job ID: 187893 Job Start: Tue Oct 2 00:10:27 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 31 Dec 2016 - GDAS0p5

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Job ID: 187941 Job Start: Tue Oct 2 00:11:32 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 1 Jan 2017 - GDAS0p5

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Job ID: 188001 Job Start: Tue Oct 2 00:12:45 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 2 Jan 2017 - GDAS0p5

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Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
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Job ID: 188411 Job Start: Tue Oct 2 00:22:30 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 11 Jan 2017 - GDAS0p5

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Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
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Job ID: 120465 Job Start: Wed Oct 3 05:10:41 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 22 Jan 2017 - GDAS0p5

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Job ID: 117897 Job Start: Wed Oct 3 01:52:28 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 23 Jan 2017 - GDAS0p5

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Job ID: 117905 Job Start: Wed Oct 3 01:53:32 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 24 Jan 2017 - GDAS0p5

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Job ID: 194500 Job Start: Tue Oct 2 05:00:43 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 25 Jan 2017 - GDAS0p5

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Job ID: 194533 Job Start: Tue Oct 2 05:01:40 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 26 Jan 2017 - GDAS0p5

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Job ID: 194558 Job Start: Tue Oct 2 05:02:30 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 27 Jan 2017 - GDAS0p5

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Job ID: 194562 Job Start: Tue Oct 2 05:03:17 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 28 Jan 2017 - GDAS0p5

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Job ID: 194605 Job Start: Tue Oct 2 05:04:12 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 29 Jan 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 7: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

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Job ID: 194632 Job Start: Tue Oct 2 05:05:02 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 30 Jan 2017 - GDAS0p5

118 120 122 124 126 128 130 132 134

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 31 Jan 17

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Job ID: 194677 Job Start: Tue Oct 2 05:06:03 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 31 Jan 2017 - GDAS0p5

115 120 125 130 135

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 15 Mar 17

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Job ID: 120591 Job Start: Wed Oct 3 05:14:07 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 15 Mar 2017 - GDAS0p5

124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 16 Mar 17

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Job ID: 117937 Job Start: Wed Oct 3 01:54:53 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 16 Mar 2017 - GDAS0p5

126 127 128 129

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 17 Mar 17

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Job ID: 117950 Job Start: Wed Oct 3 01:56:28 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 17 Mar 2017 - GDAS0p5

124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 18 Mar 17

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Job ID: 194711 Job Start: Tue Oct 2 05:06:56 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 18 Mar 2017 - GDAS0p5

122 124 126 128

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 19 Mar 17

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Job ID: 194740 Job Start: Tue Oct 2 05:08:00 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 19 Mar 2017 - GDAS0p5

124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 20 Mar 17

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Job ID: 194768 Job Start: Tue Oct 2 05:09:03 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 20 Mar 2017 - GDAS0p5

114 116 118 120 122 124 126 128 130

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 21 Mar 17

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Job ID: 194798 Job Start: Tue Oct 2 05:10:07 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 21 Mar 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 8: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

126 128 130 132 134

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 24 Mar 17

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Job ID: 120639 Job Start: Wed Oct 3 05:16:45 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 24 Mar 2017 - GDAS0p5

122 124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 25 Mar 17

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AGL

Job ID: 117964 Job Start: Wed Oct 3 01:57:55 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 25 Mar 2017 - GDAS0p5

116 118 120 122 124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 26 Mar 17

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Job ID: 117995 Job Start: Wed Oct 3 01:59:19 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 26 Mar 2017 - GDAS0p5

114 116 118 120 122 124 126 128 130

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 27 Mar 17

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Job ID: 194843 Job Start: Tue Oct 2 05:11:13 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 27 Mar 2017 - GDAS0p5

116 118 120 122 124 126 128 130 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 28 Mar 17

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Job ID: 194900 Job Start: Tue Oct 2 05:12:21 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 28 Mar 2017 - GDAS0p5

124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 29 Mar 17

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Job ID: 194933 Job Start: Tue Oct 2 05:13:24 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 29 Mar 2017 - GDAS0p5

124 125 126 127 128 129 130 131

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Job ID: 194995 Job Start: Tue Oct 2 05:14:41 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 30 Mar 2017 - GDAS0p5

120 122 124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 31 Mar 17

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Job ID: 195009 Job Start: Tue Oct 2 05:17:59 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 31 Mar 2017 - GDAS0p5

118 120 122 124 126 128 130 132 134

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 01 Apr 17

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AGL

Job ID: 195059 Job Start: Tue Oct 2 05:22:49 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 1 Apr 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 9: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

116 118 120 122 124 126 128 130 132

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Job ID: 195079 Job Start: Tue Oct 2 05:28:46 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 2 Apr 2017 - GDAS0p5

120 122 124 126 128 130 132 134

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 03 Apr 17

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Job ID: 195115 Job Start: Tue Oct 2 05:33:07 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 3 Apr 2017 - GDAS0p5

127 128 129 130 131 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 04 Apr 17

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Job ID: 195126 Job Start: Tue Oct 2 05:34:06 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 4 Apr 2017 - GDAS0p5

128 130 132 134 136

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 05 Apr 17

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Job ID: 195166 Job Start: Tue Oct 2 05:35:52 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 5 Apr 2017 - GDAS0p5

126 128 130 132 134 136

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 06 Apr 17

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Job ID: 195220 Job Start: Tue Oct 2 05:36:53 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 6 Apr 2017 - GDAS0p5

120 122 124 126 128 130

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 07 Apr 17

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Job ID: 195276 Job Start: Tue Oct 2 05:37:51 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 7 Apr 2017 - GDAS0p5

122 124 126 128 130 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 08 Apr 17

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Job ID: 195318 Job Start: Tue Oct 2 05:38:34 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 8 Apr 2017 - GDAS0p5

124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 09 Apr 17

GFSG Meteorological Data

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AGL

Job ID: 195367 Job Start: Tue Oct 2 05:39:27 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 9 Apr 2017 - GDAS0p5

118 120 122 124 126 128 130 132

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Job ID: 195418 Job Start: Tue Oct 2 05:40:24 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 10 Apr 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
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114 116 118 120 122 124 126 128 130 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 11 Apr 17

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Job ID: 195459 Job Start: Tue Oct 2 05:41:22 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 11 Apr 2017 - GDAS0p5

118 120 122 124 126 128 130 132 134

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Job ID: 195517 Job Start: Tue Oct 2 05:42:43 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 12 Apr 2017 - GDAS0p5

120 122 124 126 128 130 132 134 136

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 13 Apr 17

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Job ID: 195569 Job Start: Tue Oct 2 05:43:43 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 13 Apr 2017 - GDAS0p5

127 128 129 130 131 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 14 Apr 17

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Job ID: 195608 Job Start: Tue Oct 2 05:44:44 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 14 Apr 2017 - GDAS0p5

127 128 129 130 131 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 15 Apr 17

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Job ID: 195670 Job Start: Tue Oct 2 05:45:49 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 15 Apr 2017 - GDAS0p5

126 127 128 129 130 131 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 16 Apr 17

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Job ID: 195715 Job Start: Tue Oct 2 05:46:48 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 16 Apr 2017 - GDAS0p5

122 124 126 128 130 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 17 Apr 17

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Job ID: 195776 Job Start: Tue Oct 2 05:47:49 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 17 Apr 2017 - GDAS0p5

118 120 122 124 126 128 130

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 18 Apr 17

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Job ID: 195819 Job Start: Tue Oct 2 05:48:39 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 18 Apr 2017 - GDAS0p5

118 120 122 124 126 128 130

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 19 Apr 17

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Job ID: 195867 Job Start: Tue Oct 2 05:49:48 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 19 Apr 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 11: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

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Job ID: 195921 Job Start: Tue Oct 2 05:50:36 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 20 Apr 2017 - GDAS0p5

126 128 130 132 134 136

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 25 Apr 17

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Job ID: 120732 Job Start: Wed Oct 3 05:24:09 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 25 Apr 2017 - GDAS0p5

124 126 128 130 132 134

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 26 Apr 17

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Job ID: 118016 Job Start: Wed Oct 3 02:00:39 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 26 Apr 2017 - GDAS0p5

118 120 122 124 126 128 130 132 134 136

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 27 Apr 17

GFSG Meteorological Data

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ers

AGL

Job ID: 118026 Job Start: Wed Oct 3 02:01:55 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 27 Apr 2017 - GDAS0p5

120 122 124 126 128 130 132 134

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32

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0 500 1300

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 28 Apr 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 195988 Job Start: Tue Oct 2 05:51:46 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 28 Apr 2017 - GDAS0p5

123 124 125 126 127 128 129 130

26

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 29 Apr 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 196069 Job Start: Tue Oct 2 05:53:00 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 29 Apr 2017 - GDAS0p5

127 128 129 130 131

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26

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 30 Apr 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 196134 Job Start: Tue Oct 2 05:54:09 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 30 Apr 2017 - GDAS0p5

126 127 128 129 130

25

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0 500

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0005/01

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 01 May 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 196218 Job Start: Tue Oct 2 05:55:32 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 1 May 2017 - GDAS0p5

126 128 130 132 134

24

26

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0 500

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0005/02

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 02 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 196285 Job Start: Tue Oct 2 05:56:43 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 2 May 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 12: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

126 128 130 132 134 136

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0005/03

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 03 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 196349 Job Start: Tue Oct 2 05:57:56 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 3 May 2017 - GDAS0p5

123 124 125 126 127 128 129

25

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6 506

1306

0005/04

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 04 May 17

GFSG Meteorological Data

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Met

ers

MSL

Job ID: 196455 Job Start: Tue Oct 2 05:59:25 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 4 May 2017 - GDAS0p5

122 124 126 128 130

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0 500

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0005/05

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 05 May 17

GFSG Meteorological Data

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26

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Met

ers

AGL

Job ID: 196535 Job Start: Tue Oct 2 06:00:51 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 5 May 2017 - GDAS0p5

124 126 128 130 132

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26

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0 500

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0005/06

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 06 May 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 196638 Job Start: Tue Oct 2 06:02:23 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 6 May 2017 - GDAS0p5

124 126 128 130 132

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500 1000 1500

0 500

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0005/07

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 07 May 17

GFSG Meteorological Data

Sour

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26

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Met

ers

AGL

Job ID: 196742 Job Start: Tue Oct 2 06:03:33 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 7 May 2017 - GDAS0p5

126 128 130 132

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0 500

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0005/08

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 08 May 17

GFSG Meteorological Data

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AGL

Job ID: 196860 Job Start: Tue Oct 2 06:05:14 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 8 May 2017 - GDAS0p5

122 124 126 128 130 132

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0 500

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0005/09

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 09 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 196919 Job Start: Tue Oct 2 06:06:33 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 9 May 2017 - GDAS0p5

116 118 120 122 124 126 128 130 132

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 10 May 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 196940 Job Start: Tue Oct 2 06:07:21 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 10 May 2017 - GDAS0p5

126 127 128 129 130 131

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 11 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 196996 Job Start: Tue Oct 2 06:08:54 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 11 May 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 13: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

124 126 128 130 132 134

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 12 May 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 197017 Job Start: Tue Oct 2 06:09:41 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 12 May 2017 - GDAS0p5

118 120 122 124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 13 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197048 Job Start: Tue Oct 2 06:10:42 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 13 May 2017 - GDAS0p5

123 124 125 126 127 128 129

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0005/14

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 14 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197065 Job Start: Tue Oct 2 06:11:40 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 14 May 2017 - GDAS0p5

126 127 128 129 130 131

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0 500

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0005/15

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 15 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197103 Job Start: Tue Oct 2 06:12:38 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 15 May 2017 - GDAS0p5

124 126 128 130 132 134

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0 500

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0005/16

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 16 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197149 Job Start: Tue Oct 2 06:13:38 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 16 May 2017 - GDAS0p5

124 126 128 130 132

26

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0 500 1300

0005/17

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 17 May 17

GFSG Meteorological Data

Sour

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Met

ers

AGL

Job ID: 197195 Job Start: Tue Oct 2 06:14:38 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 17 May 2017 - GDAS0p5

125 126 127 128 129 130 131 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 18 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197231 Job Start: Tue Oct 2 06:15:38 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 18 May 2017 - GDAS0p5

128 129 130 131

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 19 May 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 197281 Job Start: Tue Oct 2 06:16:36 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 19 May 2017 - GDAS0p5

128 130 132 134

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 20 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197303 Job Start: Tue Oct 2 06:17:33 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 20 May 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 14: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

128 130 132 134 136 138

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 21 May 17

GFSG Meteorological Data

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AGL

Job ID: 197357 Job Start: Tue Oct 2 06:18:35 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 21 May 2017 - GDAS0p5

128 130 132 134 136 138 140

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 22 May 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197397 Job Start: Tue Oct 2 06:19:38 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 22 May 2017 - GDAS0p5

127 128 129 130 131 132

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0 500 1300

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 15 Jun 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 120830 Job Start: Wed Oct 3 05:31:21 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 15 Jun 2017 - GDAS0p5

127 128 129 130 131

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0 500 1300

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 16 Jun 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 118097 Job Start: Wed Oct 3 02:09:41 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 16 Jun 2017 - GDAS0p5

128 130 132 134 136 138

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0 500 1300

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 17 Jun 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 118103 Job Start: Wed Oct 3 02:10:53 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 17 Jun 2017 - GDAS0p5

128 130 132 134

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 18 Jun 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197463 Job Start: Tue Oct 2 06:20:39 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 18 Jun 2017 - GDAS0p5

120 122 124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 19 Jun 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 197526 Job Start: Tue Oct 2 06:21:40 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 19 Jun 2017 - GDAS0p5

118 120 122 124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 20 Jun 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 197564 Job Start: Tue Oct 2 06:22:38 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 20 Jun 2017 - GDAS0p5

118 120 122 124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 21 Jun 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 197618 Job Start: Tue Oct 2 06:23:37 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 21 Jun 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 15: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

120 122 124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 22 Jun 17

GFSG Meteorological Data

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AGL

Job ID: 197664 Job Start: Tue Oct 2 06:24:33 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 22 Jun 2017 - GDAS0p5

122 124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 23 Jun 17

GFSG Meteorological Data

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AGL

Job ID: 197707 Job Start: Tue Oct 2 06:25:32 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 23 Jun 2017 - GDAS0p5

124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 24 Jun 17

GFSG Meteorological Data

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AGL

Job ID: 197739 Job Start: Tue Oct 2 06:26:36 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 24 Jun 2017 - GDAS0p5

120 122 124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 25 Jun 17

GFSG Meteorological Data

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AGL

Job ID: 118112 Job Start: Wed Oct 3 02:12:06 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 25 Jun 2017 - GDAS0p5

118 120 122 124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 26 Jun 17

GFSG Meteorological Data

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AGL

Job ID: 118129 Job Start: Wed Oct 3 02:13:24 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 26 Jun 2017 - GDAS0p5

120 122 124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 27 Jun 17

GFSG Meteorological Data

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AGL

Job ID: 197763 Job Start: Tue Oct 2 06:27:51 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 27 Jun 2017 - GDAS0p5

124 126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 28 Jun 17

GFSG Meteorological Data

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AGL

Job ID: 197797 Job Start: Tue Oct 2 06:28:50 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 28 Jun 2017 - GDAS0p5

126 128 130 132 134 136

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 29 Jun 17

GFSG Meteorological Data

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28.2

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ers

AGL

Job ID: 197808 Job Start: Tue Oct 2 06:29:37 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 29 Jun 2017 - GDAS0p5

122 124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 30 Jun 17

GFSG Meteorological Data

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AGL

Job ID: 197827 Job Start: Tue Oct 2 06:30:25 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 30 Jun 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 16: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

126 128 130 132

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 01 Jul 17

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Job ID: 197868 Job Start: Tue Oct 2 06:31:27 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 1 Jul 2017 - GDAS0p5

126 128 130 132 134

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 02 Jul 17

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AGL

Job ID: 197897 Job Start: Tue Oct 2 06:32:29 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 2 Jul 2017 - GDAS0p5

122 124 126 128 130 132 134 136 138

16

18

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 03 Jul 17

GFSG Meteorological Data

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AGL

Job ID: 197926 Job Start: Tue Oct 2 06:33:27 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 3 Jul 2017 - GDAS0p5

127.0 127.2 127.4 127.6 127.8 128.0 128.2 128.4 128.6

26.4

26.6

26.8

27.0

27.2

27.4

27.6

500 1000 1500

0 500

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0007/18

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 18 Jul 17

GFSG Meteorological Data

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AGL

Job ID: 121007 Job Start: Wed Oct 3 05:41:07 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 18 Jul 2017 - GDAS0p5

124 125 126 127 128 129

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26

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0007/19

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 19 Jul 17

GFSG Meteorological Data

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AGL

Job ID: 118130 Job Start: Wed Oct 3 02:14:40 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 19 Jul 2017 - GDAS0p5

125 126 127 128 129 130

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25

26

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 20 Jul 17

04 UTC 20 Jul GFSG Forecast Initialization

Sour

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AGL

Job ID: 118144 Job Start: Wed Oct 3 02:15:56 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 20 Jul 2017 - GDAS0p5

126.5 127.0 127.5 128.0 128.5 129.0

25.5

26.0

26.5

27.0

500 1000 1500

0 500

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0007/21

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 21 Jul 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 197966 Job Start: Tue Oct 2 06:34:33 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 21 Jul 2017 - GDAS0p5

126 127 128 129

26

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 22 Jul 17

GFSG Meteorological Data

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AGL

Job ID: 198002 Job Start: Tue Oct 2 06:35:36 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 22 Jul 2017 - GDAS0p5

125 126 127 128 129 130

26

27

28

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 23 Jul 17

GFSG Meteorological Data

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26

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Met

ers

AGL

Job ID: 198046 Job Start: Tue Oct 2 06:36:18 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 23 Jul 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 17: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

125 126 127 128 129

26

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 24 Jul 17

GFSG Meteorological Data

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AGL

Job ID: 198080 Job Start: Tue Oct 2 06:37:03 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 24 Jul 2017 - GDAS0p5

126 127 128 129

26

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 25 Jul 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 198109 Job Start: Tue Oct 2 06:37:49 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 25 Jul 2017 - GDAS0p5

127.8 128.0 128.2 128.4 128.6 128.8 129.0 129.2 129.4

26.0

26.2

26.4

26.6

26.8

27.0

500 1000 1500

0 500

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0007/26

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 26 Jul 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 198144 Job Start: Tue Oct 2 06:38:36 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 26 Jul 2017 - GDAS0p5

127 128 129 130 131

25

26

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 27 Jul 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 198176 Job Start: Tue Oct 2 06:39:36 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 27 Jul 2017 - GDAS0p5

128 129 130 131

26

27

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500 1000 1500 2000 2500

0 500 1300

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 28 Jul 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 198197 Job Start: Tue Oct 2 06:40:39 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 28 Jul 2017 - GDAS0p5

122 124 126 128 130 132 134 136

18

20

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 29 Jul 17

GFSG Meteorological Data

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Met

ers

AGL

Job ID: 198244 Job Start: Tue Oct 2 06:41:37 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 29 Jul 2017 - GDAS0p5

122 124 126 128 130 132 134

20

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 30 Jul 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 198255 Job Start: Tue Oct 2 06:42:21 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 30 Jul 2017 - GDAS0p5

126 127 128 129 130 131 132

24

25

26

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0 500

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0007/31

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 31 Jul 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 198320 Job Start: Tue Oct 2 06:43:17 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 31 Jul 2017 - GDAS0p5

127 128 129 130 131 132

26

27

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 01 Aug 17

GFSG Meteorological Data

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26

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Met

ers

AGL

Job ID: 198346 Job Start: Tue Oct 2 06:44:15 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 1 Aug 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 18: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

126 128 130 132 134

26

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 02 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198371 Job Start: Tue Oct 2 06:45:14 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 2 Aug 2017 - GDAS0p5

124 126 128 130 132

26

28

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 03 Aug 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 198403 Job Start: Tue Oct 2 06:46:11 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 3 Aug 2017 - GDAS0p5

126 128 130 132 134 136

26

28

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 04 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198423 Job Start: Tue Oct 2 06:47:00 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 4 Aug 2017 - GDAS0p5

120 122 124 126 128

24

26

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 05 Aug 17

GFSG Meteorological Data

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Met

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AGL

Job ID: 198454 Job Start: Tue Oct 2 06:47:42 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 5 Aug 2017 - GDAS0p5

118 120 122 124 126 128 130

20

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 06 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 121168 Job Start: Wed Oct 3 05:46:25 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 6 Aug 2017 - GDAS0p5

120 122 124 126 128 130

22

24

26

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0 500

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0008/07

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 07 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 118156 Job Start: Wed Oct 3 02:16:55 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 7 Aug 2017 - GDAS0p5

120 122 124 126 128 130

22

24

26

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 08 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 118170 Job Start: Wed Oct 3 02:18:04 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 8 Aug 2017 - GDAS0p5

118 120 122 124 126 128 130

20

22

24

26

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500 1000 1500 2000 2500

0 500 1300

0008/09

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 09 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198495 Job Start: Tue Oct 2 06:48:31 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 9 Aug 2017 - GDAS0p5

114 116 118 120 122 124 126 128 130

20

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0 500 1300

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 10 Aug 17

GFSG Meteorological Data

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Job ID: 198525 Job Start: Tue Oct 2 06:49:33 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 10 Aug 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 19: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

122 124 126 128 130

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 11 Aug 17

GFSG Meteorological Data

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Job ID: 198541 Job Start: Tue Oct 2 06:50:36 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 11 Aug 2017 - GDAS0p5

120 122 124 126 128

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 12 Aug 17

GFSG Meteorological Data

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Job ID: 198579 Job Start: Tue Oct 2 06:51:25 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 12 Aug 2017 - GDAS0p5

122 124 126 128

24

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 13 Aug 17

GFSG Meteorological Data

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Job ID: 198600 Job Start: Tue Oct 2 06:52:17 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 13 Aug 2017 - GDAS0p5

124 126 128 130

24

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 14 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198627 Job Start: Tue Oct 2 06:53:13 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 14 Aug 2017 - GDAS0p5

122 124 126 128 130

22

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 15 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198668 Job Start: Tue Oct 2 06:54:18 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 15 Aug 2017 - GDAS0p5

124 125 126 127 128 129

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0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 16 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198704 Job Start: Tue Oct 2 06:55:17 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 16 Aug 2017 - GDAS0p5

125 126 127 128 129

25

26

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 17 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198720 Job Start: Tue Oct 2 06:56:00 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 17 Aug 2017 - GDAS0p5

127.0 127.2 127.4 127.6 127.8 128.0 128.2 128.4 128.6

26.6

26.8

27.0

27.2

27.4

27.6

500 1000 1500

0 500

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 18 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198751 Job Start: Tue Oct 2 06:56:49 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 18 Aug 2017 - GDAS0p5

127 128 129 130

26

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 19 Aug 17

GFSG Meteorological Data

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AGL

Job ID: 198793 Job Start: Tue Oct 2 06:57:48 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 19 Aug 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 20: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

128 130 132 134 136

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18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 20 Aug 17

GFSG Meteorological Data

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Job ID: 198823 Job Start: Tue Oct 2 06:58:47 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 20 Aug 2017 - GDAS0p5

128 130 132 134 136

26

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NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 08 Oct 17

GFSG Meteorological Data

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Job ID: 121307 Job Start: Wed Oct 3 05:50:56 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 8 Oct 2017 - GDAS0p5

128 130 132 134 136 138

24

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28

30

500 1000 1500

0 500

1300

0010/09

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 09 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 118194 Job Start: Wed Oct 3 02:21:01 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 9 Oct 2017 - GDAS0p5

118 120 122 124 126 128 130

26

28

30

32

34

500 1000 1500 2000 2500 3000 3500

0 500 1300

0011/24

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 24 Nov 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 121503 Job Start: Wed Oct 3 05:57:41 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 24 Nov 2017 - GDAS0p5

128 130 132 134 136 138

24

26

28

30

500 1000 1500 2000

0 500

1300

0010/10

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 10 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 118209 Job Start: Wed Oct 3 02:22:23 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 10 Oct 2017 - GDAS0p5

128 130 132 134 136

24

26

28

500 1000 1500 2000 2500

0 500 1300

0010/11

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 11 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 198860 Job Start: Tue Oct 2 07:00:11 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 11 Oct 2017 - GDAS0p5

128 130 132 134 136

24

26

28

500 1000 1500

0 500

1300

0010/12

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 12 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 198882 Job Start: Tue Oct 2 07:01:11 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 12 Oct 2017 - GDAS0p5

128 130 132 134 136

22

24

26

28

500 1000 1500

0 500

1300

0010/13

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 13 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 198911 Job Start: Tue Oct 2 07:02:07 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 13 Oct 2017 - GDAS0p5

126 128 130 132 134 136

22

24

26

28

500 1000 1500

0 500

1300

0010/14

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 14 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 198940 Job Start: Tue Oct 2 07:03:05 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 14 Oct 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 21: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

128 130 132 134 136

22

24

26

28

500 1000 1500

0 500

1300

0010/15

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 15 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 198964 Job Start: Tue Oct 2 07:04:06 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 15 Oct 2017 - GDAS0p5

128 130 132 134

24

26

28

500 1000 1500 2000

0 500

1300

0010/16

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 16 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 198990 Job Start: Tue Oct 2 07:05:19 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 16 Oct 2017 - GDAS0p5

128 130 132 134

24

26

28

500 1000 1500

0 500

1300

0010/17

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 17 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199039 Job Start: Tue Oct 2 07:06:17 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 17 Oct 2017 - GDAS0p5

128 129 130 131 132 133

25

26

27

28

500 1000 1500

0 500

1300

0010/18

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 18 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199069 Job Start: Tue Oct 2 07:07:01 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 18 Oct 2017 - GDAS0p5

128 129 130 131 132 133

25

26

27

28

500 1000 1500

0 500

1300

0010/19

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 19 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199094 Job Start: Tue Oct 2 07:08:03 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 19 Oct 2017 - GDAS0p5

128 130 132 134

24

26

28

500 1000 1500 2000 2500

0 500 1300

0010/20

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 20 Oct 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199128 Job Start: Tue Oct 2 07:08:57 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 20 Oct 2017 - GDAS0p5

126 127 128 129 130 131 132 133

26

27

28

29

30

500 1000 1500

0 500

1300

0011/25

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 25 Nov 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 118230 Job Start: Wed Oct 3 02:24:28 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 25 Nov 2017 - GDAS0p5

126 128 130 132 134

22

24

26

28

500 1000 1500

0 500

1300

0011/26

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 26 Nov 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 118244 Job Start: Wed Oct 3 02:25:35 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 26 Nov 2017 - GDAS0p5

126 128 130 132 134

26

28

30

500 1000 1500

0 500

1300

0011/27

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 27 Nov 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199151 Job Start: Tue Oct 2 07:09:50 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 27 Nov 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 22: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

122 124 126 128 130 132 134

24

26

28

30

500 1000 1500 2000 2500 3000

0 500 1300

0011/28

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 28 Nov 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199182 Job Start: Tue Oct 2 07:11:35 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 28 Nov 2017 - GDAS0p5

126 128 130 132

26

28

500 1000 1500 2000 2500

0 500 1300

0011/29

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 29 Nov 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199213 Job Start: Tue Oct 2 07:12:22 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 29 Nov 2017 - GDAS0p5

128 129 130 131

26

27

28

500 1000 1500

0 500

1300

0011/30

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 30 Nov 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199253 Job Start: Tue Oct 2 07:13:05 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 30 Nov 2017 - GDAS0p5

120 122 124 126 128 130 132 134 136

26

28

30

32

34

500 1000 1500 2000

0 500

1300

0012/01

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 01 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199289 Job Start: Tue Oct 2 07:13:53 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 1 Dec 2017 - GDAS0p5

122 124 126 128 130 132 134

26

28

30

32

500 1000 1500 2000 2500

0 500 1300

0012/02

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 02 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199327 Job Start: Tue Oct 2 07:14:56 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 2 Dec 2017 - GDAS0p5

124 126 128 130 132 134

24

26

28

30

500 1000 1500 2000

0 500

1300

0012/03

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 03 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199381 Job Start: Tue Oct 2 07:16:35 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 3 Dec 2017 - GDAS0p5

118 120 122 124 126 128 130

26

28

30

32

34

500 1000 1500 2000 2500 3000

0 500 1300

0012/04

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 04 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199423 Job Start: Tue Oct 2 07:17:16 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 4 Dec 2017 - GDAS0p5

112 114 116 118 120 122 124 126 128 130

26

28

30

32

34

36

500 1000 1500 2000 2500 3000 3500

0 500 1300

0012/05

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 05 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199458 Job Start: Tue Oct 2 07:18:16 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 5 Dec 2017 - GDAS0p5

120 122 124 126 128 130

26

28

30

32

1000 2000 3000

0 500 1300

0012/06

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 06 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199493 Job Start: Tue Oct 2 07:19:16 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 6 Dec 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 23: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

124 126 128 130

24

26

28

30

500 1000 1500 2000 2500

0 500 1300

0012/07

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 07 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199538 Job Start: Tue Oct 2 07:20:02 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 7 Dec 2017 - GDAS0p5

115 120 125 130

25

30

35

500 1000 1500 2000 2500

0 500 1300

0012/08

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 08 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199557 Job Start: Tue Oct 2 07:20:42 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 8 Dec 2017 - GDAS0p5

118 120 122 124 126 128 130 132 134

26

28

30

32

34

500 1000 1500 2000 2500 3000

0 500 1300

0012/09

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 09 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199590 Job Start: Tue Oct 2 07:21:40 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 9 Dec 2017 - GDAS0p5

120 122 124 126 128 130

24

26

28

30

500 1000 1500 2000 2500

0 500 1300

0012/10

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 10 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199611 Job Start: Tue Oct 2 07:22:21 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 10 Dec 2017 - GDAS0p5

114 116 118 120 122 124 126 128 130

26

28

30

32

34

36

500 1000 1500 2000 2500 3000

0 500 1300

0012/11

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 11 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199649 Job Start: Tue Oct 2 07:23:04 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 11 Dec 2017 - GDAS0p5

118 120 122 124 126 128 130 132

26

28

30

32

34

500 1000 1500 2000 2500

0 500 1300

0012/12

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 12 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199667 Job Start: Tue Oct 2 07:23:44 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 12 Dec 2017 - GDAS0p5

120 122 124 126 128 130 132 134 136

26

28

30

32

34

36

500 1000 1500 2000

0 500

1300

0012/13

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 13 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199710 Job Start: Tue Oct 2 07:24:41 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 13 Dec 2017 - GDAS0p5

120 122 124 126 128 130 132

26

28

30

32

34

1000 2000 3000

0 500 1300

0012/14

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 14 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199769 Job Start: Tue Oct 2 07:25:37 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 14 Dec 2017 - GDAS0p5

128 129 130 131

26

27

28

500 1000 1500 2000

0 500

1300

0012/15

18 12 06

NOAA HYSPLIT MODEL Backward trajectories ending at 0600 UTC 15 Dec 17

GFSG Meteorological Data

Sour

ceat

26

.87

N 1

28.2

5 E

Met

ers

AGL

Job ID: 199795 Job Start: Tue Oct 2 07:26:18 UTC 2018Source 1 lat.: 26.866953 lon.: 128.248468 hgts: 0, 500, 1300 m AGL Trajectory Direction: Backward Duration: 24 hrs Vertical Motion Calculation Method: Model Vertical Velocity Meteorology: 0000Z 15 Dec 2017 - GDAS0p5

Akane Yamakawa
Figure SI 2. Air-mass back trajectories of 24-h duration (continue)
Page 24: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

Table S1: Concentrations and isotopic compositions of GEM and wind directions during sampling periods at CHAAMS. Air-mass back trajectories of total run time of 24-hours were calculated for 3 days before sampling, and during sampling using the NOAA HYSPLIT model. (N: North, S: South, W: West, E: East, NW: Northwest, NE: Northeast, SW: Southwest, SE: Southeast, MD*: Multiple directions)

�Hg concentration and Hg isotopic compositions �Wind directions

No.

Sampling Date GEM δ202Hg Δ199Hg Δ200Hg Δ191Hg

Before Sampling During Sampling

Start End ng/m3 ‰ ‰ ‰ ‰

72-hour 48-hour 24-hour Day 1 Day 2 Day 3 Day 4

1 2016/12/19 2016/12/22 1.3 -0.05 -0.24 -0.19 -0.23

N N E E E E SE

2 2016/12/22 2016/12/25 1.6 -0.07 -0.20 -0.07 -0.19

E E E SW NW NC, SC E

3 2016/12/25 2016/12/28 1.4 -0.22 -0.29 0.02 -0.18

SW NW NC, SC E E NE N

4 2016/12/28 2016/12/31 1.0 -0.14 -0.25 -0.15 -0.25

E E NE N NW N NE

5 2016/12/31 2017/1/3 1.3 -0.34 -0.18 0.05 -0.15

N NW N NE NW, N E, W N, NW

6 2017/1/3 2017/1/6 1.7 -0.26 -0.16 -0.05 -0.15

NE NW, N MD N, NW NE, NW NE MD

7 2017/1/6 2017/1/9 1.7 -0.19 -0.19 -0.10 -0.19

N, NW NE, NW NE MD MD MD NW

8 2017/1/9 2017/1/12 1.0 -0.09 -0.20 -0.09 -0.12

MD MD MD NW N N, NW N, NW

9 2017/1/25 2017/1/28 1.0 0.16 -0.32 -0.13 -0.22

NW NW N, NW N NE, NW E E

10 2017/1/28 2017/1/31 0.9 0.41 -0.21 0.01 -0.17

NW N N, NW N, NW SE NW, W N, NW

11 2017/3/18 2017/3/21 1.7 0.79 -0.13 -0.04 -0.12

N NE S, SW S W, NW SW NW

12 2017/3/27 2017/3/30 1.4 -0.09 -0.18 -0.09 -0.16

NE, N N, NW NW NW NW SE, SW SE, W

13 2017/3/30 2017/4/2 1.4 -0.41 -0.07 0.04 -0.17

NW NW SE, SW SE, W S, SW NW NW

14 2017/4/2 2017/4/5 1.1 -0.39 -0.14 -0.01 -0.17

SE, W S, SW NW NW N NE SE

15 2017/4/5 2017/4/8 1.3 -0.03 -0.14 -0.07 -0.15

NW N NE SE SE SE, W S

16 2017/4/8 2017/4/11 1.5 -0.30 -0.12 0.00 -0.10

SE SE SE, W S SW SW NW, W

17 2017/4/11 2017/4/14 1.7 -0.15 -0.26 -0.07 -0.07

S SW SW NW, W NW N E, SE

18 2017/4/14 2017/4/17 1.7 -0.32 -0.24 -0.14 -0.12

NW, W NW N E, SE SE, S SE, SW S

19 2017/4/17 2017/4/20 2.1 -0.28 -0.16 -0.03 -0.07

E, SE SE, S SE, SW S NW, W NW S

20 2017/4/28 2017/5/1 0.9 -0.25 -0.22 -0.07 -0.14

E SE, S N N NW MD SE, SW

21 2017/5/1 2017/5/4 1.0 -0.20 -0.15 -0.07 -0.11

N NW MD SE, SW E, S SE, SW E

Page 25: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

22 2017/5/4 2017/5/7 1.4 -0.06 -0.19 -0.06 -0.13

SE, SW E, S SE, SW E S, SW SW, NW N, E

23 2017/5/7 2017/5/10 1.6 -0.42 -0.18 -0.01 -0.11

E S, SW SW, NW N, E E, W S NW, W

24 2017/5/10 2017/5/13 1.7 -0.15 -0.15 -0.02 -0.13

N, E E, W S NW, W MD S SW

25 2017/5/13 2017/5/16 1.4 -0.22 -0.22 -0.01 -0.13

NW, W MD S SW W MD NE

26 2017/5/16 2017/5/19 1.3 -0.40 -0.23 -0.11 -0.18

SW W MD NE NE, N N NE

27 2017/5/19 2017/5/22 1.4 -0.51 -0.20 -0.07 -0.11

NE NE, N N NE E E E

28 2017/6/18 2017/6/21 1.2 -0.36 -0.16 -0.05 -0.16

NE, N MD E NE SE, SW S, SW S, SW

29 2017/6/21 2017/6/24 1.3 -0.22 -0.23 -0.09 -0.14

NE SE, SW S, SW S, SW S, SW S S

30 2017/6/27 2017/6/30 0.9 -0.12 -0.19 -0.03 -0.21

SW SW SW SW S SE S, SW

31 2017/6/30 2017/7/3 1.4 0.01 -0.29 -0.10 -0.24

SW S SE S, SW S, SE SE S

32 2017/7/21 2017/7/24 2.3 -2.15 -0.05 0.04 -0.05

NW, W SW, S SW SW NW, SW NW NW

33 2017/7/24 2017/7/27 2.6 -1.77 -0.08 -0.02 -0.13

SW NW, SW NW NW NW MD SE

34 2017/7/27 2017/7/30 1.6 -1.76 -0.08 -0.02 0.03

NW NW MD SE E SE, SW S

35 2017/7/30 2017/8/2 2.4 -1.47 -0.05 0.01 -0.04

SE E SE, SW S SE NE NE

36 2017/8/2 2017/8/5 2.1 -1.46 -0.09 0.01 -0.10

S SE NE NE N NE W

37 2017/8/9 2017/8/12 2.2 -1.70 -0.04 0.02 -0.05

SW, W SW, W SW SW SW, W SW, W W

38 2017/8/12 2017/8/15 2.2 -1.73 0.00 0.00 0.03

SW SW, W SW, W W SW, W SW SW

39 2017/8/15 2017/8/18 2.1 -2.01 -0.09 0.00 -0.14

W SW, W SW SW SW, W SW MD

40 2017/8/18 2017/8/20 2.3 -2.01 -0.08 -0.05 -0.14

SW SW, W SW MD NE E, SE E

41 2017/10/11 2017/10/14 2.1 -1.26 -0.09 -0.07 -0.03

NE, E E E E E SE SE

42 2017/10/14 2017/10/17 2.0 -1.14 -0.09 -0.06 -0.08

E E SE SE SE E E

43 2017/10/17 2017/10/20 1.6 -1.38 -0.14 -0.04 -0.10

SE SE E E E E E

44 2017/11/27 2017/11/30 1.7 -0.73 -0.16 -0.04 -0.11

NW NE SE NE MD MD NE, E

45 2017/11/30 2017/12/3 1.7 -0.53 -0.13 -0.07 -0.15

NE MD MD NE, E N MD MD

46 2017/12/3 2017/12/6 1.3 -0.62 -0.11 -0.03 -0.07

NE, E N MD MD NW, N NW NW

47 2017/12/6 2017/12/9 1.5 -0.38 -0.21 -0.04 -0.18

MD NW, N NW NW MD NW NW

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48 2017/12/9 2017/12/12 1.4 -0.56 -0.19 -0.07 -0.13

NW MD NW NW MD NW NW

49 2017/12/12 2017/12/15 1.5 -0.36 -0.12 -0.01 -0.12

NW MD NW NW N N, NW NE

*When it is difficult to determine the direction of the trajectory, the result is written as MD.

Page 27: Supporting Information to: Investigation of Mercury Emission … · 2019-04-03 · Supporting Information to: Investigation of Mercury Emission Sources Using Hg Isotopic Compositions

Figure S3. Ox concentrations at the monitoring stations (*preliminary results fromhttp://soramame.taiki.go.jp). From late July to August (gray bars), the relativelysmall peaks indicate low δ202Hg values in the GEM samples.

month

Ox

(ppm

)

12 121 2 3 4 5 6 7 8 9 10 11