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Transcript of Pressure effect on electrical conductivity of Mott insulator “Ba 2 IrO 4 ” Shimizu lab. ORII...
![Page 1: Pressure effect on electrical conductivity of Mott insulator “Ba 2 IrO 4 ” Shimizu lab. ORII Daisuke 1.](https://reader035.fdocuments.us/reader035/viewer/2022070415/56649ef15503460f94c02cd1/html5/thumbnails/1.jpg)
Pressure effect on electrical conductivity of Mott insulator “Ba2IrO4”
Shimizu lab. ORII Daisuke
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Contents
• Introduction : H. Okabe et al., Phys. Rev. B 83, 155118(2011)
Mott insulatorBa2IrO4 Mottness
Structure Magnetic property
High-pressure effect
• Motivation• Research• Summary
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Mott insulatorEE
Introduction
EF
largeOn-site coulomb interaction U
MetalKitaoka-sensei’s lecture
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U
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Ba2IrO4 : MottnessIntroduction
Iridium 5d5eg
t2g
Crystal field SO coupling
5d
Insulator ??
Metal??
4B. J. Kim et al., PRL 101, 076402 (2008)
EEF
EEF
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Ba2IrO4 : structure
• Same structure with high-Tc materialsEx.) Sr-La-Cu-O, Ba-La-Cu-O, etc…
• 2 dimensionalityThe effect of
spin fluctuationstrongly appears.
Introduction
The interaction is weaker for lower dimension.
Flat IrO2 square
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Ba2IrO4 : magnetic property
• Spin fluctuationBoth oh the magnetic moments are reduced by the spin fluctuation.
• Antiferromagnetic order Neel temperature TN is similar.
Magnetic moment(at low temperature)
TN
Ba2IrO4 0.34 μB/Ir atom 240 K
La2CuO4 0.40 μB/Cu atom 220 K
D. Vaknin et al., Phys. Rev. Lett. 58, 2802 (1987)
Ba2IrO4 will be superconductor…?
Introduction
Ba2IrO4 La2CuO4
compare
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High-pressure effectPressure
Electronic states change!
Transitions• Structural transition• Magnetic transition• M-I transition
etc…
I’m particularly interested in superconducting transition.
Introduction
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Motivation
It is expected thatsuperconductivity will be observed
in Ba2IrO4.
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How to make high pressureMeasurement
• Electrical resistance; 4-terminal method
• Pressure Ruby fluorescence method
• Temperature
Research
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V+
V-
I+ I-
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ResultResearch
Metallic behavior
12~23GPa Insulator behavior
10
~10K
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Discussion• M-I transition
Research
But the superconductivity phase was not observed down to 10K.
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E E
?
H. Okabe et al., Phys. Rev. B 84, 115127 (2011)
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Summary
• M-I transition was observed at 25 GPa.
• But superconductivity was not observed.
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