PHYS 342/555PHYS 342/555 Condensed Matter in a …...Condensed Matter in a Nutshell Instructor: Dr....
Transcript of PHYS 342/555PHYS 342/555 Condensed Matter in a …...Condensed Matter in a Nutshell Instructor: Dr....
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PHYS 342/555PHYS 342/555Condensed Matter in a Nutshell
Instructor: Dr. Pengcheng DaiProfessor of PhysicsProfessor of Physics
The University of Tennessee(Room 407A Nielsen 974 1509)(Room 407A, Nielsen, 974-1509)
Lecture room 314 Nielsen Chapter 8: F i f d t lChapter 8: Fermi surfaces and metals
Lecture in pdf format will be available at:http://www phys utk eduhttp://www.phys.utk.edu
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Fermi surfaces and metals
FThe Fermi surface is the surface of constant energy in space.
The electrical properties of the metal are determined by the shapek
of the Fermi surface.
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Reduced zone scheme'
' 'For a Bloch function written as ( ) ( ), with '
outside the first Brillouin zone, we have ' .
ik rk kr e u r k
k k G
'' ' '
outside the first Brillouin zone, we have .
( ) ( ) ( ) ( ) ( )ik r ik r iG r ik rk k k k k
k k G
r e u r e e u r e u r r
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Periodic zone scheme
kThe energy of a band is periodic function in reciprocal
lattice: . This is known as the periodic zone scheme.
k k G
as the periodic zone scheme.In a simple cubic lattice, the dispersion has form:dispersion has form:
2 (coscos cos
k xk ak k
)cos cosy zk a k ).a
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Construction of Fermi surfaces2The equation of the zone boundaries is 2 0 and isk G G
The equation of the zone boundaries is 2 0 and is
satisfied if terminates on the plane normal to at the
k G G
k G
midpoint of .G
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Nearly Free electrons
The interaction of the electron with the periodic potential ofh l h b d ithe crystal causes energy gaps at the zone boundaries.
Almost always the Fermi surface will intersect zone boundariesperpendicularly.The crystal potential will round out sharp corners in the Fermi surfaces.The total volume enclosed by the Fermi surface depends onlyon the electron concentration.
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Make a plot of the first two Brillouin zones of a primitive rectangular two-dimensional lattice with axes, , 3 .a b a
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Electron orbits, hole orbits, and open orbits
An electron on the Fermi surface will move in a curve on the Fermi surface because it is a surface of constant energythe Fermi surface, because it is a surface of constant energy.
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Tight banding method for energy bands
Tight banding approximation deals with the case in which the ovelap of atomic wave functions is enough to requirethe ovelap of atomic wave functions is enough to requirecorrections to the picture of isolated atoms, but not so
h t d th t i d i ti i l tmuch as to render the atomic description irrelevant.
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Assuming that in the vicinity of each lattice point the fullAssuming that in the vicinity of each lattice point the fullHamiltonian can be approximated by of a single atom located at the lattice point If is a bound level
atH H natom located at the lattice point. If is a bound level
of for an atom at the origatH
in, . ( ) ill b ll h d di t f th d
at n n n nH E r
will be very small when exceeds a distance of the orderof the lattice constant.
r
To calculate the extreme case in which the crystal differsfrom , ( ), where (at at
HH H H U r U
) contains allrcorrections to the atomic potential of the crystal. If satisfies , then it will also satisfy the crystal
n
at n n nH E
Schrodinger equation if ( ) vanishes wherever ( )does not. To p
nU r r
reserve Bloch condition, we must have
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n
n
Each atomic level ( ) would yield levels in the
periodic potential, with wave function ( ), for each
r N
r R
np p ( )
of the sites in the lattice.
( ) ( )ik R
N R
r e r R
n ( ) ( ),
The Bloch condition is satisfi
nR
r e r R ed ( ) ( ).ik Rr R e r
The Bloch condition is satisfied ( ) ( ).The energy bands have no difference from the energy of
of the atomic level regardless of the value of
r R e r
E k
of the atomic level, , regardless of the value of .Consider the general form of the wave function:
nE k
( ) (ik Rr e r ).
RR
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If ( ) ( ) is nonzero but small,( ) should be quite close to the atomic wave function ( ).
n
n
U r rr r
( ) ( ). Then we have crystal Schrodinger equationn
n nn
r b r
( ) ( ( )) ( ) ( ) ( )
MultipatH r H U r r k r
*ly by the atomic wave function ( ), integratem r
* * *
over all , consider
( ) ( ) ( ( )) ( ) ( ) ( ) ,m at at m m m
r
r H r dr H r r dr E r r dr
* *( ) ( ) ( ) ( ) ( ) ( ) .
C id i th thm m mk E r r dr r U r r dr
lit f th t i f tiConsidering the ortho*
normality of the atomic wave function,
( ) ( )m n nmr r dr
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W i i l i h d i hWe arrive at an eigenvalue equation that determines the
coefficients ( ) and the Bloch energies ( ):nb k k
*
0
( ) ( ) ( ) ( ) ik Rm m m m n n
n R
k E b k E r r R e dr b
*( ) ( ) ( )m n nn
r U r r dr b
*(m
0
) ( ) ( ) .
The first term contains integral of the form
ik Rn n
n R
r U r r R e dr b
*
The first term contains integral of the form
( ) ( )m nr r R dr
Our assumption of well-localized atomic levels mean that the above term is small compared to unity.
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We assume that the integral in the third term is small, since they also contain the product of two atomic wavesince they also contain the product of two atomic wave functions centered at different sites. Finally, we assume that the second term on the right is small because we expectthat the second term on the right is small because we expectthe atomic wave functions to become small at distances large enough fo the periodic potential to deviate appreciablylarge enough fo the periodic potential to deviate appreciablyfrom the atomic one.
0Therefore, ( ) if is not smmk E b all or vice versa.
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Application to an s-band arising form a single atomic s-levelatomic s-level
If all the coefficient are zero that for a single atomic -level,
( ) ik R
b s
R e
( )( ) , where is the energy of the
1 ( )i l l d
s sik R
R ek E E
R e
*
atomic -level and
( ) ( ) , ( ) ( ) ( )
s
U r r dr R r r R dr ,
*( ) ( ) ( ) ( ) .
Since is an -level, ( ) only depends on magnitude of
R r U r r R dr
s r
Since is an level, ( ) only depends on magnitude of
and ( ) ( ). Since ( ) ( ), ( ) ( ).If we assume that only nearest-neighbor separations give
s r
r R R U r U r R R
If we assume that only nearest-neighbor separations give appreciable overlap integrals, we have
( ) ( ) cosk E R k R
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( ) ( ) cossn n
k E R k R
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For FCC crystal, the 12 nearest neighbors of the origin are
( 1, 1,0), ( 1,0, 1), (0, 1, 1).a a aR
( , , ), ( , , ), ( , , )2 2 2
For ( , , ), ( , ), , , ; , ; , .2x y z i jak k k k k R k k i j x y y z z x
2
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Consider ( ) ( , , ) has full cubic symmetry,
( ) is the same constant for all 12 of the vectors
U r U x y z
R
( ) is the same constant for all 12 of the vectors.
1 1 1 1( ) 4 (cos cos cos cos2 2 2 2s x y y z
R
k E k a k a k a k a
*
1 1cos cos ), 2 2z xk a k a
1 1
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*( ) ( , , ) ( , , ) (R x y z U x y z x 1 1, , ) .2 2
a y a z dr
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Measuring the Fermi surfaceg
Fermi surface measurements require pure single crystal at lowtemperat res and is freq entl perform in er strong magnetictemperatures and is frequently perform in very strong magneticfields. The shape of the Fermi surface is intimately involved in the transport coefficients of a metal as well as in the equilibriumin the transport coefficients of a metal as well as in the equilibriumand optical properties. The most powerful method to deducethe Fermi surface geometry is the de Haas van Alphen effectthe Fermi surface geometry is the de Haas-van Alphen effect.
/dM dH/ , Landau accounted the
ill ti i f
dM dH
oscillations in free electron theory.
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The change in 1/ through a singleperiod of oscillation, 1/ , was
HH
determined by:1 2 1e
where is any extremal cross-sectione
e
H c AA
area of the Fermi surface in a planenormal to the magnetic field.
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Th d H Al h ff i i di iThe de Haas-van Alphen effect is an indicationof the failure of the semiclassical model. The f il i h th i l i l thfailure arises whenever the semiclassical theorypredicts closed orbits for the electron motion
j t d l di l t th fi ldprojected on a plane perpendicular to the field.When this happens, the energies of motion
di l t ti dHperpendicular to are quantized.H
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Free electrons in a uniform magnetic fieldg
The orbital energy levels of an electron in a cubic box with sidesof length parallel to the - - and -axes are determined inL x y zof length parallel to the , , and axes are determined inthe presence of a uniform magnetic field along the -directionby two
L x y zH z
quantum numbers and :kby two
2
2
quantum numbers, and :
1( ) , .2 2
z
z z c c
k
eHk km mc
2 2
runs through all nonmagnetic integers, and takes on the same values as in the absence of a magnetic field:
z
m mck
g2 / for any integral z zk n L n .
The energy of motion perpendicular to the field, which wouldz
2 2 2
gy p p ,be ( ) / 2 if no field were present, is quantized in
steps of ( / ) This is orbit quantizationx yk k m
eH mc
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csteps of ( / ). This is orbit quantization.c eH mc
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Semi-classical motion in a uniform magnetic field
In the semiclassical equation of motion:
1 ( ) ( ) 1k d k
1 ( ) ( ) 1( ) , ( ) ( ) .
Electrons move along curves given by the intersection of
k d kv k e v k Hdt ck
g g ysurfaces of constant energy with planes perpendicularto the magnetic field.g
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Origin of the oscillatory phenomena
Most electronic properties of metals depend on the density of levels
at the Fermi energy, . It follows that will be singular whenever the value of causes an extramal orbit on the Fermi surface
F Fg gH
4
to satisfy the quantization condition ( + ) ( ).1 2 1 . 1.34 10 / .
e FA Ae e K G
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. 1.34 10 / .
e F B
K GH c A mck
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Dai/PHYS 342/555 Spring 2012 Chapter 9-43
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Dai/PHYS 342/555 Spring 2012 Chapter 9-44