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Optical and ESR Characterization of Transition Atoms in...
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i 993 i C d Ykh 1 naryompounsooama , , t l u pp.1143 8 8 4 3, - 2 3 . fT nAtmsnCAIS 2 u i o io t i rans KA l LJ - ies. it ur l b a eI , he h h ff t ecargeranserro lt e b i mt he dt an, are i ternares or hll se - ilt rvaenca an an lt novaen an lf taso i Sb or nb df mo dt nb dd - t enca l nova lf tasomo i ke i l - onor l tt aencesaes an ht eype t ne mi dv t ns trea l her i dt onsuner t t era ma me d h an l aenc h l ta i b r softe v ebdtote3 - orac - onor tt an h l eresu - hecon t - d一 n l eve i l p l e 色 一 ds tl sof3 oU yofAg dT , y l tzoog h ec turean LCl ru . t i vers E n Tk oy l tzoogy, h ec hi eron t l f t eemenso ) A lt a- ht os - demarca ( y i d t onoeepenerg lt ea - ionspec i lb t caasorp hi t erongroupop , t f tyo i mpur hI dM ppl 2(993 ppl Op dESRCh no dT yofT T t t onao dERp 2S ht m( ii rans t il ld di t ngecrysasopew , t esuya mi t t onao io nr mp n3po Rs hl cacoge ii t orgnae l l ecua an gi lc n te t es , i t t aracerza t t rucure do t Sid ii t tt ernaryemconucorrans , i yr mo ro hl acop t Su F l acu S ) S il caan E trum, co t eragona 1 n t C fT t n on ernaryan . . h Vl3 yso . . t t ecen yearsernary h P . t P 9 roc. J A J pn.. C llii t rysazn I A hC e i t t esn u lS ii hl bi tt esneacvaencesaeeng t h i i esempur 2 t i f onso i tt veconcenra h lt erea f l t ttt erenvaencesaes, i hid er it n i t cearepresen t ii mpur TAi h tt a hb f d aseenoun t idI e. ih b d t aveeensu , N FC d neoan ,,, iVCM r ,, , iT group e ,.. kesposs ic i h onsw , t hma - g ma O d un hb d ean i l l eve hF eer t f mp mi nt ies it ur he i nerge it se io r it onza i d gan b d serve h h how n av l b a ao epara t fl o i n t specr ii transon h w erea Th me samo gtel ma dhebeeno ,ael nT di sT eIIs stei ne sOft ions i tt rena he A li eves i t rcao e h io it os dT noftedma nl nt le Tb a n i rze iesaresu d tu h te f tso l eresu Th ESRs mma di by t u ) d oun 3 , mp ur f eror b as . h i rze h ■ean u it w av l t t rysagrow w h d i ereas opng ig. h I w in hf dMnh eenp medd gtec hbyteCVT nF 1 eh esmma dteo ion ilb t ca asorp t p d - ic f h orw 2 , A u i ons hT e t f terso Ai nC lS hd n use h l t eexerna S l aues i p i t qecv h t s daswe , il e f i t nec ntot lla ee es nv di WA A K I H b r l tasan i b r d3do NIS i b k ouyu i nr hh d t eoscompoun t hb d f eangapo it n ll eve hF i eerm t f tono h ii epos d dt t epenenon h te h O on. l ta i b r sofTA i nteo rh 2+- io dt conuc - hll se - d O S hC eu t AI 2C h lf t ecrysaso ii es t i ur nt in ll t conro gt ) iesan it ur dby 2 io f dt o conuc l tas i b r b or t i i onspar t i trans yf k 3 es ic ose i h onsw , co t mp dof3 hma io t h i epos no den d i 1 J 4 apan , 8 iTk ogane oyo , K igan l do dM 2 993) 41 , ay Ri eceve ( VN , O N t t pecra. Oun il caan t p i h cangeno dESRs mp dwihTA imp e a f tureo b m have ing h tt esar C C r oan , , , i t t nsn il see , h s suc ddi a n haTiⅤ dNi eencrrido gt me ot ix t eer h i t avere h i cangn ) T f o by We dtod Aimp 1 gt t C ld t rysasope S hC eu t f AI 2 hTAi dwi mp ′ ft onsorw T l f vaueso - heg Ai oo o h o hi ess t yn ftec n 3+-TA2 +a t i opn l trya h b speresor io ih t ysoc f tt erena ki e i l - i t cepor ga i pb me nd mo yd gwihd mp d an. l vaenc h te eb f to io lt ea h f ranse i t e .. a h carg ban T et rt A l+ , ep dgplnr ntoRe po io lt ea i h l t ecrysa t if axso - hec h l sown ft o III, gt nr o use t ns l t t uenee i t s me dfrs O S u h t f i opn D go eC AI 2 C i ton i rans sTA 至, C 3 AxE s OIgor , T A S i k t asua K - mb pme C lh t rysasav lng 一 ter S S eena muhi ot ml hi erpro i C esu . mi AI 2 ,w hhsbeenr yf dt d t ue oun db mi eena ep ) il t caproper l S ec t t neres l nescence nl mi gd u t ecen Ho llt nC AI ea 2 i t nearop grow c - s ing l non h l t oou in h a tt ttt rac ic lu dere te d t nescenan h wevera , h b ave i nares n i ons ih gree g lu gr b l rose i a a hb ean t h f t ecenero dgpwillgno t snear - er f eec h h t io t lf eveo h nerg to li d t evesnrouce , i n h t f t se iii vcn energ t a he he i ince S i nqu l l eve ecnbeudtomo rtemo nofteF mi nt yo ee yl ed t. yl dbyt trong oemits d n lu o i tera dtobeap ema lfrb ea iv t erspec hose f eec ap. an h ot ro eb Ad it es t ene l mp dtoe hi h ic h tyw , ft dg et tw ec foun l cos - ht eer t f ero h f ereorecan , dt an, is h tt ae l vaence harge feren i nl lofd tc d( )s soft eve io t - - e a a hb ean t in dgpcnb - are ft eec - in - - Her i - lS hCA eu t if eso t roper db Aions. T y l li d t evesnrouce ) i ton JJ eve F i t pecrum erm , AIB ht eype t d f oun so dt conucors e a an h ie it ur sinteb dgp ofsmi la ica h t eop T :C 2 S A u S J D t F dga ban dt es h i ew WO Y E K mp dit s oun co mary ebeen l d t socae io t l l i evepos ec ni d - d i t conucors e ,.. e b eoserve iesca , it ur nb dinsmi 1) d ii v- dt onuc in ･ 仙e ma ne ns nr - hF eer 触e dbyt Th t t gne rca de he h hroug esonans t s tt ae ll evepa harge i p lt ecro h yi mi sse ht ma n ic, nce . rayoftec ds softed energ lt t eecronsas df eec l di taan , , ′para ion t rca lt pi crys h te - h t cargerans he i lt onsreae , t i trans f tt aeso fl i t pesoeecronc y h t en carge Tw ds ot dtotTA f t nso t t rea l her t proper he ma me p ty - t ensae hl dp ycmp o ig h t i b i h x h tec e(ESR) tom io t i rans na t rree h t nes e , d are , S u in i ld ncu T ( ( A)imp gC AI 2) eepo Ha kap roc - A h in e f t ereore, ma i t nea h l e eT yted yd gd hi em i f mt onsro t h l i i t t eeecroncrans it e .. fl o i n d一 n hl l eeveso n ionsa t i trans imp mo gt f3 ma dofTA s ion. it za l rea i evce l l eve Fer f io t i epos no mi ill a nerg t n or r i ito onza i l t snova l eve h nerg in io t i prox d trouce l ld t eves eno , ma ni df TA.Th de yl saeesse gtei ne on. T h te Ai Fer he mi t ht a ) 2 s daswe , il e f h f l t ecysa t h f f t eeeco lla ions t f i t errans byt , - d d euce l i eeas f ero C ons a , enu i tonan. T or N ince b oserve , l l iTb sa h t ponens h i tesp fro nHami Th mb 〟 df Ai nb yd mt es t t nesrucurecom 丘 - on ec he l l eve hF eer t mi nt f d oun - rca re tt encesa l a ac h i i eseons t l vaenc i f onso ll t econroe e tt cenra t Th es ne hv ea ob dbyt e h io lt ea i l t t oscrysa h t f a ban 1 8 4 dgpo eh nr ntotedma iv lt rea he onsan o ) i ( tt aes fTA i dt . S 2 - ' f no io t h i epos - h h t ecargerans 一 ii rg - he f rro ooccu mt f ht a ose io t tt nerprea d ounsareco o uc ernar o easo i tt aes l l ecua 1 b ence an ). i ton Ther nfrshani nist mo ro ds nt ycmp mp do h te t sva per p h in d espon gtoteu mo - he S - d llo h3 e oun hht eosco t f mp dtot ieve i d i gansorvceversa 2 . i bl ernaresaree hl e i i ons t o it pur f i t errans yintot ) T nt dt - t por a o T h te lf taso i b r l b vaence an t mae do do A in(cce ta h i t pooexc ke i l orr l ta b r sc i
Transcript of Optical and ESR Characterization of Transition Atoms in...
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