Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects
description
Transcript of Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects
![Page 1: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/1.jpg)
M. Kartsovnik 22.04.23
Magnetic field induced charge-density-wave transitions:
the role of orbital and Pauli effects
Dieter Andres, Werner Biberacher and Karl Neumaier Walther- Meißner-Institut, Garching, Germany
Harald Müller European Synchrotron Radiation Facility, Grenoble, France
Natalia Kushch Institute of Problems of Chemical Physics, Chernogolovka, Russia
Mark Kartsovnik
Walther-Meißner-Institut, BADW, Garching, Germany
![Page 2: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/2.jpg)
M. Kartsovnik 22.04.23
Outline
-(BEDT-TTF)2KHg(SCN)4: layered crystal structure, Fermi surface, etc.
Influence of magnetic field on the charge-density wave (CDW)
– Pauli paramagnetic effect;
– orbital effect
Field-induced CDW (FICDW) in -(BEDT-TTF)2KHg(SCN)4 under
pressure:
B layers;
tilted fields: Commensurate Splitting effect
Summary
![Page 3: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/3.jpg)
M. Kartsovnik 22.04.23
-(BEDT-TTF)2KHg(SCN)4: basic features
CDW formation
at 8 K
very low
!!
2D Fermi surface
Nesting instability
of the Fermi surfaceQ
||(300 K) 30 – 100cm;
/|| ~ 104 105;
||(300 K)/ (1.4 K) 102
T. Mori et al., 1990
![Page 4: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/4.jpg)
M. Kartsovnik 22.04.23
0.0 0.2 0.4 0.6 0.8 1.00.0
0.2
0.4
0.6
0.8
1.0
1.2
1.4
TCDW/TCDW(0)Theory: D. Zanchi et al., PRB 1996;
P. Grigoriev&D.Lyubshin , PRB 2005
0.0 0.2 0.4 0.6 0.8 1.0
0.0
0.5
1.0
1.5
2.0
TCDW/TCDW(0), exp
Phase diagram of -(BEDT-TTF)2KHg(SCN)4
P. Christ et al., JETP Lett. 2000
~ 23 T
suppresses CDW
Spin splitting deteriorates the nesting conditions for a CDW
Q+
Q-
Q- < Q+
B
Pauli effect (isotropic)
![Page 5: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/5.jpg)
M. Kartsovnik 22.04.23
4( vt + t ’ ) / F
ky
c
kx
~ t’/ v F
-c
Orbital effect (B || z)
requires an imperfectly nesting FS:
)2cos(2)cos(2)( )( yyyyx katkatk k
)0'( tTT cc In magnetic field:
zFy Bv
e
dt
dk
;
zFyc Bvae
y ~ 1/Bz
electrons become
effectively more 1D
lB = 2vF/
c
y =
ay(4
t / c
)
Real space orbit:
![Page 6: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/6.jpg)
M. Kartsovnik 22.04.23
D. Zanchi et al.,
PRB 1996
Orbital effect (B || z)
0 2 4 6 8 100
5
10
15
20
25
30
2.3 kbar
3.6 kbar
1.8 kbar
0 kbar
B [T
]
T [K]
-(BEDT-TTF)2KHg(SCN)4
D. Andres et al.,
PRB 2001
Theory
FICDW at t’ > t’ *
due to Landau quantization of the unnested FS pocket
4( vt + t ’ ) / F
ky
c
kx
~ t’/ v F
-c
![Page 7: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/7.jpg)
M. Kartsovnik 22.04.23
The “slow oscillations”
• approximately periodic with 1/B
• appear at P Pc 2.5 kbar
FICDW: experiment; B || z
SdHo
• display a weak hysteresis
P = 3 kbar
![Page 8: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/8.jpg)
M. Kartsovnik 22.04.23
FICDW: experiment; B || z
• approximately periodic with 1/B
• appear at P Pc 2.5 kbar
• display weak hysteresis
• slightly shift with temperature
The “slow oscillations”
behaviour consistent with the FICDW scenario!!
![Page 9: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/9.jpg)
M. Kartsovnik 22.04.23
FICDW: experiment; B || z
![Page 10: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/10.jpg)
M. Kartsovnik 22.04.23
FICDW: experiment; B || z
A. Kornilov et al., PRB 2002
FICDW is weaker than FISDW due to the Pauli effect! A. Lebed, JETP Lett. 2003
FICDW
in -(BEDT-TTF)2KHg(SCN)4
FISDW
in (TMTSF)2PF6
![Page 11: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/11.jpg)
M. Kartsovnik 22.04.23
FICDW: role of the Pauli effect
N = 5 4 3 2
1
0
4N = 33
2
1
2
1
0
0
no Pauli effect (FISDW) Pauli effect on (FICDW)
Qx = 2kF + NG Qx = 2kF QP + NG
G = 2eayBz/h
QP = 2BB/hvF
![Page 12: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/12.jpg)
M. Kartsovnik 22.04.23
FICDW: role of the Pauli effect
4N = 33
2
1
2
1
0
0
no Pauli effect (FISDW) Pauli effect on (FICDW)
Qx = 2kF + NG
A. Lebed, JETP Lett. 2003
Qx = 2kF QP + NG
G = 2eayBz/h
QP = 2BB/hvF
SDWeff
CDWeff gg
BBt c /1)(/2
![Page 13: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/13.jpg)
M. Kartsovnik 22.04.23
FICDW in a tilted field
2QP = MG
A. Lebed, JETP Lett. 2003
N = 3,4 2,3
1,2
0,1
0
Commensurate splitting (A. Bjelis et al., 1999; A. Lebed, 2003) “Spin-zero”
2QP = (M + 1/2)G
with M - integer
![Page 14: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/14.jpg)
M. Kartsovnik 22.04.23
FICDW in a tilted field: experiment
cos1
222/1
B
FP
vea
Q
GM y
Spin-zero condition:
T = 0.4 K
![Page 15: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/15.jpg)
M. Kartsovnik 22.04.23
FICDW in a tilted field: experiment
cos1
222/1
B
FP
vea
Q
GM y
Spin-zero condition:
1st CS angle1st CS angle
![Page 16: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/16.jpg)
M. Kartsovnik 22.04.23
FICDW in a tilted field: experiment
cos1
222/1
B
FP
vea
Q
GM y
Spin-zero condition:
1st CS angle1st CS angle
vF 1.2105 m/s
![Page 17: Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects](https://reader036.fdocuments.us/reader036/viewer/2022062520/568157ed550346895dc5634d/html5/thumbnails/17.jpg)
M. Kartsovnik 22.04.23
Summary
The orbital effect causes FICDW transitions in -(BEDT-TTF)2KHg(SCN)4
at pressures above Pc = 2.5 kbar
The Pauli effect, in general, weakens the FICDW instability
The interplay between the orbital and Pauli effects can be controlled by
changing the field orientation:
- the FICDW is enhanced at commensurate splitting angles
- the FICDW is suppressed at „spin-zero“ angles