M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G....

14
M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia Preliminary version of the model was described in our EURISOL Research report [http://ganil.fr/eurisol]. The code FIPRODY (FIssion PRODuct Yields calculations) has been updated by inclusion advanced version of the pre- equlibrium exiton model and neutron spectra calculations. Monte Carlo method was used to simulate the time evolution of the fission process starting from the pre-equlibrium stage of reaction.

Transcript of M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G....

Page 1: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

M3.1 JYFL fission model

Department of Physics, University of Jyväskylä, FIN-40351, FinlandV.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia

Preliminary version of the model was described in our EURISOL Research report [http://ganil.fr/eurisol]. The code FIPRODY (FIssion PRODuct Yields calculations) has been updated by inclusion advanced version of the pre-equlibrium exiton model and neutron spectra calculations. Monte Carlo method was used to simulate the time evolution of the fission process starting from the pre-equlibrium stage of reaction.

Page 2: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

The code can be used for calculation folloiwing output in the proton and neutron induced reactions at energy up to 100 MeV:

• Evaporation residues cross sections.• Pre-compound neutron and proton emission spectra.• Pre-compound proton and neutron multiplicity.• Pre-scission light charged particles (p, d, α) emission multiplicities.• Pre-scission neutron spectrum.• Post-scission light charged particle multiplicities.• Post-scission neutron spectrum.• Fragment kinetic energies.• Pre-neutron emission fragment mass yields.• Fission product mass yields.• Fission product yields for isobaric chains.• Fission product yields for elemental chains.

Page 3: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

The two-component exciton model was used for our objectives: an adequate description of the initial excitation energy distribution and composition of the compound nuclei in the neutron and proton induced fission. For description of exciton evolution process the folloing transitions are taken into account:- proton particle-hole pair creation;- neutron particle-hole pair creation;- conversion of a proton particle-hole pair into a neutron particle-hole pair;- conversion of a neutron particle-hole pair into a proton particle-hole pair; - the proton emission;- the neutron emission;-after particle emission the exciton evolution process may develop further until reaching the criteria for transition to the compound stage of the reaction;

The exciton transition cascade is ruptured at reaching one of conditions:1. exciton number reaches limited value n ≥ nmax;

;2. total life time of the exciton stage exceeds limiting value Texc ≥ Tmax which corresponds to statistical width decay;3. the number of emitted particles exceeds the lemited value Mn ≥ Mn

max or Mn ≥ Mnmax

.

Page 4: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

M5 Netron and proton induced reactions at Fermi energy domain

232Th(p, f) at Ep = 13, 20, 40, and 55 MeV

The advanced experimental setup for the multi-parameter correlation measurements consists two-arms fission fragment spectrometer CORSET, 8 DEMON neutron detectors, 3 HENDES position sensitive neutron detectors, and 12 BaF2 -detectors.

Layout of detectors is shown in after next slide. Mass-kinetic energy distributions of fission fragments, double differential neutron spectra, and mean multiplicity and energy of -rays have been measured. Preliminary date are presented in the next slides.

The neutron probe is important for estimations of excitation energy of compound nuclei and strength of nuclear friction. Particle emission at pre-compound and pre-scission stages influence on the conposition and excitation energy of the fissioning nucleus at the scission and on the phission product yields.

Page 5: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

Experimenental setup in 232Th(p, f) experiment

Page 6: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.
Page 7: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

120

140

160

180

200

220

TK

E, M

eV

Ep=55 MeVE

p=40 MeVE

p=20 MeV

Ep=13 MeV

p +232Th 233Pa

0

2

4

Yie

ld, %

60 80 100 120 140 160140

150

160

170

<T

KE

>, M

eV

60 80 100 120 140 160

60 80 100 120 140 160

60 80 100 120 140 160 180

pre-neutron fragment mass, amu

Page 8: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

10-4

10-3

10-2

10-1

100

10-4

10-3

10-2

10-1

10-4

10-3

10-2

10-1

0 4 810-4

10-3

10-2

10-1

0 4 8 12

=14.50

= 00

p(13MeV)+232Th

=29.50

= 00

=44.50

= 00

d2M

n/d

Ed

, M

eV-1st

r-1

=59.70

= 00

=89.20

= 00

=119.20

= 00

=164.00

= 00

=-14.50

= 00

neutron energy, MeV

Page 9: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

10-5

10-4

10-3

10-2

10-1

100

10-5

10-4

10-3

10-2

10-1

10-5

10-4

10-3

10-2

10-1

0 10 20 3010-5

10-4

10-3

10-2

10-1

10 20 30

=14.50

= 00

p(40MeV)+232Th

=29.50

= 00

=44.50

= 00

=59.70

= 00

=89.20

= 00

d2M

n/d

Ed

, M

eV-1st

r-1

neutron energy, MeV

=119.20

= 00

=164.00

= 00

=-14.50

= 00

Page 10: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

10-5

10-4

10-3

10-2

10-1

100

10-5

10-4

10-3

10-2

10-1

10-5

10-4

10-3

10-2

10-1

0 10 20 3010-5

10-4

10-3

10-2

10-1

10 20 30

=14.50

= 00

p(40MeV)+232Th

=29.50

= 00

=44.50

= 00

=59.70

= 00

En , MeV

=89.20

= 00

d2M

n/d

Ed

, M

eV-1st

r-1

neutron energy, MeV

=119.20

= 00

=164.00

= 00

=-14.50

= 00

Comparison between experimental and theoretical (red curve) neutron spectra

Page 11: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

60 80 100 120 140 16010-4

10-3

10-2

10-1

100

0

2

4

6

232Th(p, f), Ep/MeV

13 20 40 55

Yie

ld, %

Apre

Yie

ld, %

Page 12: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

10-4

10-3

10-2

10-1

100

101

80 100 120 140 16010-4

10-3

10-2

10-1

100

232Th(p(13 MeV), f) teory experiment

yiel

d, %

pre-neutron mass number, amu

232Th(p(40 MeV), f) theory experiment

Comparison of the calculated and experimental fragment mass di´stributions

Page 13: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

Average TKE of FF

10 20 30 40 50 60160

162

164

166

168

170

<

TK

E>

, MeV

Ep, MeV

Page 14: M3.1 JYFL fission model Department of Physics, University of Jyväskylä, FIN-40351, Finland V.G. Khlopin Radium Institute, 194021, St. Petersburg, Russia.

10 20 30 40 50 600

2

4

6

8

22.9.2005

Atot

Mn

tot

Mn

post-sc

Apre-sc

Mn

pre-sc

Mp

pre-eq

mu

ltip

licity

Ep (MeV)

232Th(p, f)

Mn

pre-eq

Calculated pre-equilibrium, pre- and post-scission neutron and proton multiplicities