Low Temperature Martensitic Transition in a Pu-Ga Alloy
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Low Temperature Martensitic Transition in a Pu-Ga AlloyTai C. Chiang
Department of Physics. University of Illinois at Uranba-Champaign
X-ray thermal diffuse scattering mapping (TDS) of phonons in Pu-Ga: Results show that the L-point soft mode in Pu-Ga does not change as the temperature is lowered toward the transition temperature. This is rather unusual and points to the collective response or instability of the 5f electronic configuration as a likely driving mechanism for the transition.
TDS patterns from a (111) grain and a (110) grain at different temperatures and the corresponding fits.
Temperaure T (arb units)
Phon
on F
requ
ency
(arb
uni
ts)
(a) First Order, Type A
(b) First Order, Type B
(c) Second Order
TCT0
TC
TC Example: TiSe2
Pu
-La-Ce
Temperaure T (arb units)
Phon
on F
requ
ency
(arb
uni
ts)
(a) First Order, Type A
(b) First Order, Type B
(c) Second Order
TCT0
TC
TC Example: TiSe2
Pu
-La-Ce
Phonon frequency as a function of temperature for different types of transitions.