A major purpose of the Techni- the broadest dissemination ...

16
cal the ble A major purpose of the Techni- Information Center is to provide broadest dissemination possi- of information DOE’s Research and Development contained in Reports to business, industry, the academic community, and federal, state and iowll governments= Although a small portion of this report is not reproducible, it is being made available to expedite the availability of information on the research discussed herein.

Transcript of A major purpose of the Techni- the broadest dissemination ...

Page 1: A major purpose of the Techni- the broadest dissemination ...

caltheble

A major purpose of the Techni-Information Center is to providebroadest dissemination possi-of information

DOE’s Research and Developmentcontained in

Reports to business, industry, theacademic community, and federal,state and iowll governments=

Although a small portion of thisreport is not reproducible, it isbeing made available to expeditethe availability of information on theresearch discussed herein.

Page 2: A major purpose of the Techni- the broadest dissemination ...

TITLE FIRST DIRECT MEASUREMENTOF ALPHA-MJJONST1CK13X:IN DEUTERONTRITON -- MUON-CATALYZEDI’LIS1ON

M. A. Paciotti, O. K. Baker, J. N. Brmibury, J. S. Cohtin.M. Leon, H. R. Maltrud, L. N. Sturgess (UiNL); S. E. .Joncs,P. Li, L. M. Rees. E. V. Sheeley, J. K. Shurtleff, S. F.

AUTHOW) Taylor (Brigham Young University); A. N. Anderson {I>ahoResearch); A. J. Caffrey, J. Znbriskie (I[lilhl} NationalEnglneerlng Lilbor;ltory); F. B. Brooks, J. D. Daviefi,B. .]. I’ylc, (:. T. A. Squler (University of Birmingham);A. Bert in, M. ilru~chi, M. Piccinini, A. Vitnlc, A. ZOCC(J1l(Uniwrsity (If Bolognn -- Italy); V. R. Born. C. W. E. Viln

Eijk, H. dt’ Ilililn (De]ft University of Technol,lgy): (;. H.Eiltl)ll (Rlltll~*rl”ord-Applcmtl~n L;]horatc)ry)

MASTER

~~~~[~~~~ LosAlanlos,NewMexico87545Los Alamos National Laboratory

:11.KI’”II!III:IIN “1 1,,1 . I., l!”llmlwl IV *rim, lmmnw, ?l

About This Report
This official electronic version was created by scanning the best available paper or microfiche copy of the original report at a 300 dpi resolution. Original color illustrations appear as black and white images. For additional information or comments, contact: Library Without Walls Project Los Alamos National Laboratory Research Library Los Alamos, NM 87544 Phone: (505)667-4448 E-mail: [email protected]
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FIRST DIRECT MEASUREMENT of a – P STICKING in dt – PCF

M.A. Paciotti, O.K. Baker, J.N. Bradbury, J.S. Cohen, M. Leon,H.R. Maltrud, L.L. Sturgess,

Los Alamos Nation~ La~oratory, LOS Alamos, N .M.,

S.E. Jones, P. Li, L.M. Rees, E.V. Sh4y, J.K. Shurtleff, S. F. Taylor,

Brigham Young University, Provo, Utah,

A.N. Anderson,

Maho Research, Boise, Idaho,

A.J. Caffrey, J.M. Zabriskie

Idaho National Engineering Laboratory, Idaho Falls, Idaho

F.B. Brooks, J.D. Davies, B,J. Pyle, G.T. A. Squier,

University of Birmingham, ~hi]ton, England

A. Bertin, M. Bruschi, M. Piccinini, A. Vitale, A. Zoccoli,

University of Bologna, Bologna, Italy

V.R, Born, C.W. E. van Eijk, H. de Haan,

Delft University of Technology, and

C. H. Eaton,

Rutklerford- Appleton Laboratory,

Didcot, Oxfordshirr.

ABSTRACT

Both ( np )+ and a particles hav~ been ohscrved in coinciclrnce with fusion

ueutrone in a gaseous D – T target at 2.8 x 10 3 liquid-hydrogen density. The

initial muon sticking probability in muon-catalyzrd d -– i fusion, mewured di-rectly for the firot time, is (0.80 -+ 0.15 + 0.12 syfitcmatic)?% in agreenmnt with

‘stanclnrd’ theoretical calculations. However, thio ll~msulrd valur does not sup-

port tlmw theories thnt invokr oprcial mechanisms to altrr the initial sticking

Valurm

IN’I’ROI)[J (! ’1’ION”

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The present paper describes t,]le fir5t direct Ineasurement of the a – p stick-

ing probability, using a low dellsit,y (~ 10–3 /hd) D – 2’ mixture.12 As such,

it comes very close to measuring the initial Stickillgprobability in dt – ~CF.Extension of the this work is presently tlnderway at Rutherford- Appleto~~ Lab-

oratory ( RAL).13

oL_J5-.Jc

W4.—

N

v

Fig. 1.

F:

WI,W2:1:s:

Beryllium target flask, 6.4 cm diamdcr, 7.6 cm long;

cylindrical walls are 1.5 ll]n~ thick; contaiils D T,C’t = 0.4.

I.5 micron mylar wi-’dows aluminizd 1600 ~ on 7’2 siclr.

Purr iridium ‘() ’-ring 8ealing the target window.

Silicon surfam Imrricr rtctect.o., 1000 lllm2, 100 Inicrons thick.

M ! ,!’d2,M~~1sn!l t~!~%<~p~ CCiiiiitF4S, ea,’li 1.6 :illll thick. .. . .. .. . ,

N: Nrutron co~lnter, FIicron liquid scintillate ( F3(!-SO1 ), 12.7 crn

in dialnetrr nnd 12.7 cnl in depth; 1.6 mm vrt. o counter i~l fnmt..

11: I)ottd Iinr indicates poletip of I k(~ i}~rtll~t]rl]t magnetic firld.(~: Smondnry container for 1)2, 121 v(JulllP, Al wnils, l,ucitr Ii{l,

all senln Viton ‘() ’-rings.

W3,W4: Ilemt treated Al henil~ entrance MI(I exit wind{}ws, ().13 mm thick.

1[: I)dm-tor htmmingt sedcd, mold, mId Itltwemt)le; r{~l~taitls 1)2.

M: M{}{lrrat(]r for ~lowil~g (If)wtl 60 hleV/c Ii I)emtll.

v; (!llmrKefl I)articlr vrt.() {.{jllllt.rr.

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The CONCEPT of the LAMPF EXPERIMENT

The ( ,lP)+ ions Produced by “sticking” events and the a-particles formed

in the remaining 99 + 70 majority of events are detected in coiucidencc with the

14.1 ~JeV neutron and are easily se~arab]e by range ill the low pressure D – T

gas; the density is dictated by the very limited ranges of these ions. The fact

that the ions are produced at 180° frox~i the neutrons is useful for background

r*jection. Triggers due to (p-, prt) and (p-, ph ) captures in the target flask are

substantially suppressed since the cilarged particle is Ilot similarly correlated in14 Beryllium, chosen for its good properties in containi]lgangle with the neutron .

tritiunl and its very low n]uo~-capture prddility, is the best target IIlaterial for

use in the LAMPF beam structure. The full p– beam is directed on the targci

to achieve an adequate event rate; many muons are therefore present in t,Iie

target at one time, and there is then ah-nest no possibility to measure the fusion

tilne with respect to the muon arrival titne. (This wiil be possible using the

RAL pulsed muon beam. ) Even though high-Z materiah do not exhibit many

charged particles in coincidence with neutrons, the high capture probability

produces overwhelnling singles rates in both neutron and silicon detectors.

LAYOUT

Features of the setup are shown in Fig. 1. Most itnportant, the silicon

detector must be protected fron~ tritiunl beta radiation. 7’2 diffuses out through

the target window W1, lin~ited prilnari]y by the alunlinum coating, at a n~ea-

sured rate of 2.5’?lo per day and is diluted by the large volume of the secondary

container. The second window W2 then keeps this dilute mixture at a distance

from the dctrctor where the intervening Dz region is guarded by a magnetic

field, The detector housing is sea!ed except for a long pressure-equilibrating

capillary, necessary when the detector housing is cooled; cooling to – 7° C im-

proved the timing resolution fronl 3.5 to 3.0 ns. Target filling ie challenging since

tlw windows cannot support much ~.1iffercntin..l pressure; as a molecular sieve cold

trap cleans thr incoming premixed D – ‘I’ gas, D2 is adnlitta-i to the secondary

container at a rate ti:d maintains low riifkrcntial prenaure. Backgrounds arc

c“ 4 entirely with Da and normaiizeri to111PlW5111Tf! in S!? identicrd =P~=r=tiis JIU?(

incoming I[nuuns. A 2ss f) source, insertabl~ between W 1 and W2, gav - i:lcntical

energy and timing calibrations for rach apparatus.

‘1’hr character of thr LA MPF exprrilllent is revwdmi by typical rates; both

peak rmtrs during thr l,A MPF pul~c and mvcragr ratrs nre given in ‘1’nhlr 1.

( [)uring thin particular run prriod, a thin production t.argrt t-nused the rntcs to

Iw rwi~lced by n factor of 3 below n{~rl;lal. ) The netltron rntc n is taken after

15. thr n rmte incl!ldcs noise; n (~ I n) is tl]c trig~erplIlsr-shape {iiscrilllination ,

rate forlned witil a 150 ns coincidence wi(lth. ( !Icmrly tile f{lsif~ll [>roccss 1:1 nf}t

iji)w=rvnhir in either thr Ilrl]t.r(]ll or the (t sitlglefi rate.

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TABLE I. Typical rates.

RATE M1M2M3 y + n n c1 Cr”(?+??)----- ----- ----- - ----- - --- --- ----- --

Peak/s 2.6 x 106 1..5 x 104 560 1440 2.8Avtrage/s 1.4 x 104 810 30 80 0.15

SYSTEMATIC EFFECTS

The factor 4 ratio between (aP)+ and a ranges was utilized by two different.

schemes; in an earlier experiment both ions were detected concurrently, while for

the latest data, optimum detection of each ion required different fill pressures.

Table 11 compares merits and systematic effects for each method. At 650 Torr the

experiment is severely rate-limited and (at LAMPF ) background-limited. We

could not have been certain that (cr~)+ had been seen without a higher density

run. Using the dual pressure scheme, a strong (ap)+ signal is seen. However,

the usefulness of the data may be linlited by the systematic uncertainty of yield

~ scaling wit b density d, This scheme present:$ a good opportu~~ity to nleasure

stripping effects.

TABLE 11. Syst~nlatic effects.

(rip)+ and a dctcc!ed concurrently :-.

1) Single fill, # -= 1.0 x 10-3 lhd, 650 Torr.

2 ) a’s we collected from only 1/2 of target volume nearest the window.

3 ) p “- stopping distribution must be well known,

4 ) a ranges must be known very well.

.5~ ~aa impuri~ y only affecta the fusion yield ~ , not the sticking result.

6) Slightly lower stripping since (up)+ energies are higher.

7J No lp, dp diffusion effect.

R) (’f only alters the yield y.

Srparafr D T ftffs for (ay)+ and a ohcrvotion :—...—. —— .—. ——--.-— .—

1) ‘rwO fills, @ 7.6 x 10-4 (490 Turr)fr and @ -2.8 x 10 ‘3(1800 Torr)((t p)+

2 ) floth ions are c{jllectcd fronl the fl~ll targrt voluille.

4) Most ~lnccrtainty in range cance]u o{lt,

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A Monte ~Jarlo code is USefU1 for evalllating these systematic effects, b~lt

the experiment is not so ~~nlPli~ated th~t the ~ode is css~ntial to the analysis.Figure 2 displays the distributions Of fusion events in the du~-pressure schenle,

reflecting principally the nluon stol)ping distr~}~uti~n, detector solid angles, and

particle range. a-particles originating near the back of the flask fall below the

0.7 MeV threshold and a~e not detected. The code finds a 93?10 active VOIUINe,

whereas the (crp)+ active volume is 100%. According to the prescription, we

could have used about 460 Torr to avoid this correction, but we favored instead

a slightly higher density to obtain a higher x. The overall efficiency is slnall

(0.08% per stopped p-), independent of density, and, aside from the volume

correction, cancels out of the sticking result.

I’ariation in the muon stopping intensity within the target volume was

measured by counting the 5eMn activation16 of thin iron foils placed inside the

non-t ritiated target. Compared with the central maximum, the intensity falls

to 1/2 along the axis uear the wil)dow and the back wall. The predicted stop

rate in hydrogen, based on these foils, was 4.7 x 10-4 p- stopped per incichmt

p - at 490 Torr.

o 1‘u u

a 411p

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lizing the

obtained,

to the 0.7

same windows and fill gas as fusion particles, ~iood con3ist,encY was

and we conclude that the calculated range of a 3.,5-MeV a degraded

MeV’ threshold was verified to about 2 mm.

L ——~- —“~y —

26 6 -14 .:

t“ – tn (ns)

Fig. 3. Monte Carlo prediction ~or (ap )+ at 1800 Torr. Time vs energy corre-

lation is evident. The higher e:lergy (op)+’s arrive early.

Corrections for stripping are easily and accurately given by the Monte Carlo

using the energy-dependent stripping cross sections for D – T g~, aluminum,

mylar, and D2 gas. 18 Table 111 Iigts stripping for the severnl materials assuming

an average energy at each position. It can be used to amess the relative effect

of the gas and of the windows , which are approximately equal.

TABLE 111. Stripping probabilities.

STRIPPING MATERIAL STRIPPING PROBABILITY

3.9 CC? CV9. LQ T pizt!i!ezgti’i at i8il~ Torr G.5’7’O

1600” A Al coating on target window 1.3910

1.5 ntir?on mylar (argrt wtndow 4.(s%

1.() cnr [)2 at 1800 Torr 1.0%

; ,W)O A Al coatina 01: detmtor window I.1%

1.5 rnlcron mylar drtector u)itldou! 3.!)70

I.5 f-m f~z at I 800 Torr 2.1%

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the detector window or the last 1.5-c1lI D2 region. The net result after the

code has consicierecl all of the above ( stopping distribut.irm, solid angle, ener~.y

loss, stripping a! proper energies, and det.ectioll threshold) is that only 1670 of

the initially prod~lced (OP )+ are uliobserved. This effective stripping, R.ff =

0.16, is quite small considering that more eflicient strippers such as aluminum

and mylar have been introduced. Strippil,g is significantly less than that seen

when t.lle ion is allowed to stop flllly in a mediume, al]d convinces us that

initial sticking is close at hand in this direct method. Verification of strippiug

calculations could be accomplished in these experill~ent, s, for exa]nple, by testing

the effect of additional mylar. Reduced background. at RAL will also be Iwlpful.

Fusion a particles generated between W 1 and W2 could simulate ( ap )+ ●’ents;

however, C’~ is so low there that the correction to w: is estimated to be much

less than 1% of w: and is therefore neglected.

DATA

The pulse-shape discril~lil~at.iol]ls picture is given in Fig. 4 showing the

location of the cut that selects the approximately 4% neutron signal from the

remaining y‘s that arise mainly from muon-decay electrons.

The a-data are presented first. since the signal is so prominent (Fig. 5).

only the neutrons have been selcctmi, and prompt muons have been rejected.

l’he time difference between the cr-ion and the fusion neutron is plotted along

the abscissa while the ion energy is plotted along the ordinate. The box drawn

shows the region where the a’s are expected from Monte Carlo predictions. The

position of the box along the time axis cannot be known from measurement, so

the a-data themselves are used as a g~licie to positioning the box. (rip)+ ions

are also expected in this plot, but with such low rate that background masks

them.

The {aP)+ spectrum for all data taken at 1800 Torr is shown in Fig. 6,

where tile axes are the same aa in Fig. 5. A quick comparison with its con]panion

background plot shows a strong signal, but of course not as cban as the a data.

‘1’hc coincident background, which extends frotn threshold to well above the

maximum (op)+ energy, comes from from p - capture in the beryllium target

flask; protons, cieutermm, tritons, and alphas, are ~lllittal in cAnc;A-~t-- wit!;. . . . . . ..\...-

ncu t rons. Non-coincident background, in the wings of t}m time distribution,

originatm [ronl a variety of sourrcs producing singles, including srntterd n~tlons

which caunot be rr)mpletrly rejm-teri at]d products frolll p capturr in Iwryiiilllll,

poiydhyiene, and aiuminum.

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.

.

1

9U0 1000 Pulse Shape 1200 1300

Fig. 4. Neutron srparalion by pulse shape.

. .

. .. .

,..:....’.. . I

.0.,. .

It@-.+. ..:.. I:8 i :.:.. .II . ~:?. . .. . . . . “’ . ..”.’ :“

.m @ -14 -S4

t. - :. (-)

Fig. 5. 0 datn on thr IFft. 13ackgrrmnd on thr right for I/7 nllrllhrr of incident

lllll{m~.

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.. .. .:.

.;:””,.::::. .. .. .. . ..:. :,

. .::.::... .. .

- 26” a -14 .34t. - k (m)

1.”:,.... ..: .;.

. . 1-6.5

Fig. 6. The (crp)+ spectrum for all data taken at 1800 Torr. Backgrotind is

shown cm the right for 3/4 number of incident muons.

Table IV lists the raw numbers obtained from the data.

TABLE IV. Raw Data.

PRESS[JRE REGION COUNTS.----- ---- -----

1800 Torr (al<)+ 115

1800 Tow Background go

490 I’orr c? 295490 Torr Backgrmnd 3

M1.M2.M3-----

16.7 X 10g

29.1 X 109

7.2 X 10*

1.0.5x 109

PIJRITY OF D – T GAS

An anticipated source of trouble was impurities in the D – T mixture.

(See table }1. ) The mylar window precludes a high- tcmperat ure bakeout of the

target, and there just is not enough gas to overpower small fixed amounts of

contaminants as there is for the high-pressure targets .*2 The procedurr used

was to fill first to 1800 ‘Torr slid to collect ( crp) + data, then to bleed the gas

prf=m-l!m d.Qwn ~Q 4!2!2 ~.Oii afid ~dle~t a dnta. in this way, tive same gas was

~Iscd for the measurement and for the normalization. Tilne-dependrnt evolution

of contaminants from the walls by t.ritium is not prevrnteri by thin procedllrc,

b(,t nonr was evident. A second 1800 -Torr data r~ln prodilced 30Y0 nlort= (rip)+

than did the first 1800 -Torr fill when normalized to ente,.ing muons while no

changes werr evidmt in the hackgroul]d. It was not posijiblr to accot~lplish tlie

bled procedure for this till, and so confident norll~dization is hicking for Illorethan ]/2 of thr (rip)+ counts in Fig. 6. ‘1’he direction of the ohsrrvd effectis consistent with a rleanrr Illixturr being obtainr(l (or tile secolltl fill foll(~willg

tritiuul scouring of tllc surfacm occuring {Iurillg tllc first fill. t!olltalllit]ation

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of the 112 in the secondary container could also contaminate the target gas by

diffusion through the window; we expert less such impurity for a seco]ld El].

Although the increase is not statistically conclusive, its directiol~ reinforces our

belief that it is due to a change in gas properties. Consequently, only the first

set of runs at 1800 ‘1’orr were used in deriving the sticking probability, the data

appearing in Table IV. If ilnpurity did cause the change in X, we estinlat,e about

600 ppln (with the Z of nitrogeu) was present.

RESULTS

The initial sticking probability is given by

Here

Nnop

a~ = ‘—”—N#2(l – R=ff)’

(2a)

11~N. =

N~2 0.93 (26)

wht=rc nm (tIaP ) is the nurmher of doul)ly (singly) charged ions detected, Ii’<ff

is the effcctiv~’ stripping, and 0.93 the active volume for cr. N is the nul]lber

of incident ,,l~lons in eacl. case ( Ilorlllalizati(}n to the high-energy coillcidrnt

background WM SIIOWI1 to be eqllivale[lt). We assunle for now that both the

riumber of ii st0pp6d and thr yield y are prr)porti{]nal tO @. (See the next

section. ) I’he reslllt is U: = (0.80 * 0. 14)% (statistical error).

UJj ~nensllred in the 650-Tt>rrexI}erill]ellt. is (0,91 +0.3)70 (stat.lstica] error ).*9

‘“1’heerror is larger since fewer ( n~i ) + were ol)serveci in thr presence of substantial

l}ackgro~tlld.

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SYSTEMATIC UNCERTAINTY

We now examine systematic uncertainties for itenls in Table 11 listed ~nder

“.$qarate D–?’jifls jor(ap)+ andc r”. The i/L and dp diffusion distances

are limited by the muon lifetime et such low pressures and ~~~lld become sonw-

what longer due to diffusion while the atoms are ~tiil el}ithernlal. We estinlate

this distance to be about 1 cm at 490 ‘1’err, somewhat smailer than the dimen-

sions of the target. No correction is made at this time; generalization of C:ohen’s

solution to the time- deperident Boltzmann equationzo to get the spatia] eytent

would be appropriate for a good estimate.

The most important uncertainty is a conseqllmce of the use of two different

densities in making the measurements. At our densities thermalization times

equal or exceed the muon lifetime. Therefore most of the molecular formation

will occur in the epithermrd (transient) region where A4~P is rapidly changing,

and the yield x may then not scale with del~sity as assullled above. Table V

attempts to outline the scope of this problem. Tllermalizaticm tinles, a~ well

as average temperature and remaining triplet fraction at a relevant tillle t~f 2

ps (,all from ref. 20) tell us that at the lowest density the tp atoms rt=inain

hot, and the triplet quenching is not con} plete. The muon lifetime then selects

rat her different slices of the cpit hermal transient for each density. (See survey of

experinlen+rd kw-density transients in refs. 21 and 22 and calculated transient

effects in ref. 23)

TABLE V. Density Effect,

J(“ [lANTITY 490 Torr 1S00 Torr------ --------- --.------ ----------

Ilm. qitp+ 7.6 x 10-4 2.8 x 10 3

Thermafizntion time (i /1s ] .6 /1.9

,4vcragf ttmpt’r(lturc at 2 ~i.~ WOK MOh”

tp triplrt frnctio7z d 2 p.~ 0.33 0.04

Avmagr Adtp 1.5 x 108 1.3 x 108

Extrapolated q,, from rrf.31 0.77 (J.56

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here the strongest density depen~~ence is predicted at IOTVdensity. The direction

of the qls density dependence is to offset the increased formation rate exPecte(l at

the low density. In this simplified treatment, the 0.33 triplet fraction remaining

in the 49o Torr sample has little ef%ct on the conclusion; in the event that

27 the triplet fraction could approach zeroA~~ is actually larger than calculated ,

WithOUt largely affeCtillg ~he htp haled ill the table.

~onie comments are in order: 1) Expected epithernlal ellhallcelllellt Of ~dtp

makes the ql. den ty dependence more important in determining yield at Ct =

0.4. Hence the RAL experiment may find a larger optimunl C’t where the higher

yield would be welcome. 2) Xlo effects would iikely enter in a important way if

a proper evaluation over the complete epithermrd peak were clone. 3 ) Thern~al-

ization could be more rapid than reported. 4) We should pay attention to the

4*5 keeping ill mind that the lowest-densityplunging cycle rates at low density,

points (#J= l?lo) are already heavily into the epitherma! region. But simply taking

,X = q!J&/AO = 0.08/p- (450 Torr) with & nt 45/Iis gives a predicted rate f{)r

our experiment that agrees with the absolute number of muon stops in tile mix-

ture found by foil activation. Unfortunately the foil test disagrees badly (by a

factor of 2) with the nulnber of stops estimated frcm beam properties. We might

Uimerwise have hoped to bracket tl~e extent of the cpithermal enhau -emcnt at

low densities (subject to assumptions about gas purity). 5) We anticipate that

the RAL pulsed-beam data will add to the understanding of this low density

region and answrr some of the qurrtions raised by the LAMPF e~perimcnt,.

‘1’h? initial [Tf of 0.4 falls with time, anti ionization chamhm mmsurrlmmts

Indicate C’t droplwcl to 0.38 at the en(l of t!le data collection on the first 1800

‘T(}rr fill and to 0.3’7 at the end of tile 490-’1”nrr data collection. I’his snlnll ctiangr

is significant only if the optimum (~t is nluch higl:er so that 0.4 is on the rising

rdge of the AC vs (’t curve instead of ~t the plateau wll(=re we intrndml it to he.

Variations in w: depending ou cuts 11A Ilave lN-etl evalunted in tile thmis

(!( I,i19” the rllla scatter rjll~oullts to about O. Wj’/O which we add to tllc statistical

e, ror. ‘13twwd ml the relinl}ility of the abovr Rmunlp$ions, we lwlirve it ~lnlikely

that the density effect will alter W; hy ~l~orc tl~an 1:)?lo. Accor~lillgly msystrl~lrd.ic

uncertainty is quoted with the rmult: w: (0.80 + 0.15 } 0.12 syatcmatic)%

Slllmeqtlmlt cxperilllents or calculations (JI1 tile f!mlflity effect can I)e tlfml to

cflrrrct this reslllt.

‘1’ile tihO-’i’fmr si.lcking measurmm=nt, m outiinrfi ill Tmbic ii, (iOe~ not mnthin

IIncertn.itlly d~ie tO tile (Iensity efrect, all(l its u}usistcwt vallle of (0. !11 1 ().3)0/0

(stntist,icnl crr{,r) a,lfls c,,,,fi(lc,,cr to t,tlr cf,ncl,lsi,,,l.

(: ON(:I, !ISION”

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.,

theoretical calcu)ations28’2 g’30 an~! not sllpporting those theories that invoke ape.

31 132*3.$ The r~l)ortefi vdIIe containscid mechanisms to alter t.hc initial sticking

only a 16% correction to the observed sticking due to stripping. Additional ex-

periments are underway at the Rutherford-Appleton Laboratory where a high-Z

target in the pulsed nl,uon beam ptoduces lower bnckgroundg. Direct nornmliza-

tion to neutron singles, transient observation, and reactivation tests should be

possible.

ACKNOWLEDGEMENTS

We wish to thank R. H. Sherman of the Los Alamos National Laboratory

for making a test of the cleanliness ill trit.iull~ of the thin mylar coated with

aluminum. Little ?mpurity was seen in his IZaman spectronlcter, giving us con-

fidence to proceed,

This work is supported by the U. S, Departnlent of Energy Division of

Advanced Energy Projects.

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